Issue 
A&A
Volume 585, January 2016



Article Number  A98  
Number of page(s)  24  
Section  Interstellar and circumstellar matter  
DOI  https://doi.org/10.1051/00046361/201525899  
Published online  23 December 2015 
Waveletbased crosscorrelation analysis of structure scaling in turbulent clouds
^{1} I. Physikalisches Institut, Universität zu Köln, Zülpicher Strasse 77, 50937 Köln, Germany
email: arshakian@ph1.unikoeln.de; ossk@ph1.unikoeln.de
^{2} Byurakan Astrophysical Observatory, 378433 Aragatsotn prov., and Isaac Newton Institute of Chile, Armenian Branch, Armenia
Received: 13 February 2015
Accepted: 12 September 2015
Aims. We propose a statistical tool to compare the scaling behaviour of turbulence in pairs of molecular cloud maps. Using artificial maps with welldefined spatial properties, we calibrate the method and test its limitations to apply it ultimately to a set of observed maps.
Methods. We develop the waveletbased weighted crosscorrelation (WWCC) method to study the relative contribution of structures of different sizes and their degree of correlation in two maps as a function of spatial scale, and the mutual displacement of structures in the molecular cloud maps.
Results. We test the WWCC for circular structures having a single prominent scale and fractal structures showing a selfsimilar behaviour without prominent scales. Observational noise and a finite map size limit the scales on which the crosscorrelation coefficients and displacement vectors can be reliably measured. For fractal maps containing many structures on all scales, the limitation from observational noise is negligible for signaltonoise ratios ≳5. We propose an approach for the identification of correlated structures in the maps, which allows us to localize individual correlated structures and recognize their shapes and suggest a recipe for recovering enhanced scales in selfsimilar structures. The application of the WWCC to the observed line maps of the giant molecular cloud G 333 allows us to add specific scale information to the results obtained earlier using the principal component analysis. The WWCC confirms the chemical and excitation similarity of ^{13}CO and C^{18}O on all scales, but shows a deviation of HCN at scales of up to 7 pc. This can be interpreted as a chemical transition scale. The largest structures also show a systematic offset along the filament, probably due to a largescale density gradient.
Conclusions. The WWCC can compare correlated structures in different maps of molecular clouds identifying scales that represent structural changes, such as chemical and phase transitions and prominent or enhanced dimensions.
Key words: methods: data analysis / methods: statistical / ISM: structure / ISM: clouds
© ESO, 2015
1. Introduction
The interstellar medium has a complex dynamic structure on all scales (from subparsecs to at least tens of parsecs) as a result of various physical processes occurring in the multiscale turbulent cascade of molecular and atomic gas. Highresolution and high dynamic ranges of observations of emission line transitions and continuum emission of interstellar clouds provide evidence for clumpy structures on all scales (see e.g. Stutzki & Guesten 1990; RomanDuval et al. 2011) and anisotropic clouds such as shells and filaments (e.g. Men’shchikov et al. 2010; Deharveng et al. 2010). Observations of line transitions, total, and polarized continuum emission provide valuable information about physical conditions (density, temperature, magnetic field) and kinematics of a multiphase gas distributed on different scales.
The correlation between different structures measured in interstellar clouds, e.g. contours of different chemical tracers or the density, temperature, and velocity peaks, as a function of their size can be used to quantify commonalities and differences in the formation of these structures. Understanding the commonalities and differences seen in different tracers, different velocity components, or different excitation conditions as a function of scale length helps to infer the underlying physical processes in the turbulent cascade in interstellar clouds. As many processes have characteristic scales, but only show their signatures in particular tracers, to identify those scales it is essential to compare the scaling behaviour of various tracers in a same region. The characteristic scales could be: e.g. chemical transition scales (see e.g. Glover et al. 2010), when comparing molecular line maps of different species; dynamical scales, for the formation of coherent structures (Goodman et al. 1998); IR penetration scales which show up in dust continuum maps at different wavelengths (e.g. Abergel et al. 1996); ambipolar diffusion scales for dynamical coupling between ionized and neutral particles, seen when comparing maps of ionized and neutral species (McKee et al. 2010; Li et al. 2012); and dissipation scales, when comparing channel maps of individual atomic or molecular lines (Falgarone et al. 1998).
To address these issues, we use two different starting points. The wavelet analysis has been proven to be a powerful tool for detecting structures on different spatial scales in time series and in twodimensional maps. This analysis was used e.g. in the Δvariance analysis measuring the amount of structure in a molecular cloud map as a function of scale and to determine the slope of the power spectrum of the cloud scaling (Stutzki et al. 1998). A combination of a wavelet filtering with the crosscorrelation function was first proposed by NesmeRibes et al. (1995) to study solar activity. Frick et al. (2001) improved the method introducing wavelet crosscorrelation function to study the correlation between galactic images as a function of scale. This method and its modifications were successfully applied to study solar physics, ionosphere fluctuations, images of astronomical objects, and allsky surveys (e.g. Vielva et al. 2006; Liu & Zhang 2006; Tabatabaei & Berkhuijsen 2010; Roux et al. 2012; Tabatabaei et al. 2013).
These approaches, however, are not designed for recovering the displacement of structures in the data sets on scalebyscale basis and accounting for a variable noise distribution across the maps and irregular boundaries. Patrikeev et al. (2006) used an anisotropic wavelet transform to isolate spiral features in images of M 51 for different tracers and analysed their location and pitch angle as a function of radius and azimuth, but they did not crosscorrelate the features seen in different tracers. The waveletbased crosscorrelation method can be improved by inheriting the corresponding formalism from the waveletbased Δvariance analysis and combining it with the crosscorrelation analysis. To account for an uneven distribution of noise in the maps, Ossenkopf et al. (2008a, hereafter O08) implemented a weighting function in the improved Δvariance method to analyse arbitrary data sets of molecular clouds. The weighting function corrects for the contribution of data points with a varying signaltonoise ratio and allows us to perform a proper treatment of map edges, independent of their shape, and calculations in Fourier space, which speeds up the computation by making use of the fast Fourier transform. Moreover, O08 suggested an optimal shape of the wavelet filter for analysing the turbulent structures.
We make use of the advantages of weighting functions and develop a weighted wavelet crosscorrelation (WWCC) method to recover the correlation and displacement between structures of molecular clouds as a function of scale, in which no assumption about the noise or boundaries are made.
The paper is organized as follows. Section 2 introduces the Δvariance and crosscorrelation methods. The WWCC method is presented in Sect. 3. The application of the WWCC to simulated circular structures and fractal structures is described in Sect. 4. The application of the WWCC to observed emission line maps of the giant molecular cloud G 333 is presented in Sect. 5. The discussion and conclusions are presented in Sect. 6.
2. Basic theory
We consider two maps, f(x) and g(x), (x = (x,y)), weighted at each pixel by a significance function w_{f}(x) and w_{g}(x). The significance functions w_{f}(x) and w_{g}(x) characterize e.g. a variable signaltonoise ratio across the maps or can be used to treat irregular map boundaries.
2.1. Wavelet analysis to measure scaling in turbulent structures
The Δvariance measures the amount of structure in an individual map as a function of scale, thereby identifying dominant structure sizes. In this context “structure” describes the spatial variation of measured properties, i.e. a deviation from a flat or zero measurement. The amount of structure quantifies the total variation in a given map as characterized by the variance. With the Δvariance, this is evaluated as a function of the size of the structures equivalent to the power spectrum (Stutzki et al. 1998). This method represents a twodimensional generalization of the Allanvariance method (Allan 1996). The Δvariance is evaluated from the map f convolved with the wavelet ψ(1)by computing its variance (2)where the ∗ symbol represents the convolution and is the average intensity of the map. For uniform, zero average data without boundaries, this is equivalent to the wavelet power spectrum.
The wavelet is composed of a positive core, ψ_{c}, and a negative annulus, ψ_{a} i.e. (3)Core and annulus are normalized to an integrated weight of unity, so that the integral over the whole wavelet cancels to zero.
For a fast computation of the convolution in Eq. (1), Stutzki et al. (1998) used the multiplication in Fourier space, but Bensch et al. (2001) showed that this can lead to considerable errors from edge effects due to the incompatibility of the implicit assumption of periodic maps in the Fourier transform and the boundaries of real observed maps. Bensch et al. (2001) suggested a filter that changes its shape closer to the map boundaries by truncating it beyond the map edges and changing the amplitude of core and annulus to retain the wavelet normalization condition. While this improves the edge treatment, its weakness is that the convolution of the map can no longer be performed in Fourier space.
Ossenkopf et al. (2008a) suggested a modification that overcomes the edge treatment problems, and simultaneously deals with the effect of observational uncertainties and irregular map boundaries and allows for a computation in the Fourier domain. To fix the filter function, they increase the map size when the filter extends beyond the map edges and apply a zeropadding to the extended map area. The renormalization of the filter is accomplished by introducing the complementary weighting function w(x) > 0 inside the valid map and w(x) = 0 in the zeropadded region. When using a generalized weighting function 0 ≤ w(x) ≤ 1, this can characterize the significance of every individual data point, including the effects of noise and observational uncertainties. Then the map f_{p} and the weights w(x) have to be convolved separately with the positive and negative filter parts f_{c}(x,l) = f_{p} ∗ ψ_{c}(x,l), f_{a}(x,l) = f_{p} ∗ ψ_{a}(x,l), w_{c}(x,l) = w(x) ∗ ψ_{c}(x,l) and w_{a}(x,l) = w(x) ∗ ψ_{a}(x,l), and the renormalization is performed when computing the map filtered on scale l i.e. (4)When finally computing the Δvariance from the convolved map, the weights are taken into account in the sum of the variations (O08) (5)with (6)and as the weighted average of the map (7)The choice of the wavelet filter and its optimization is of great importance for the scaling analysis. For isotropic wavelets, the ratio of the core diameter to annulus diameter is the critical parameter. Ossenkopf et al. (2008a) found that both, Frenchhat, and Mexicanhat filters with a high ratio between the diameter of the annulus and the core of the filter, are preferred for measurements of the general power spectral slope, while the Mexicanhat filter with low diameter ratios is more suited to detect individual prominent scales sensitively. The Mexicanhat filter with an annulus/core diameter ratio of v = 1.5 was found to provide the best compromise, revealing the correct power spectrum slope and all spectral features. Therefore, we use the following optimal wavelet filter (Eq. (11) in O08) throughout: (8)where l is the scale of interest. The choice of the Gaussian smoothed filter is justified by the simultaneous confinement of the filter in ordinary and Fourier space. The usable range of scales l falls between 2 pixels, needed to guarantee a reasonably isotropic filter shape on a rectangular pixel grid, and about half the map size as discussed in Sect. 4.1.2. The method was proven to be a powerful tool to characterize the power spectrum of interstellar clouds (Stutzki et al. 1998; Ossenkopf et al. 2008b).
2.2. Crosscorrelation
We can compute the crosscorrelation coefficient between two images or maps f(x) and g(x) as (9)describing the degree of concordance between the maps. If all structures are shifted between the two maps, the crosscorrelation coefficient drops, but the characterization of the similarity of the two maps can be recovered when introducing a reverse offset vector t while computing the crosscorrelation. This leads to the definition of the twodimensional crosscorrelation function as a function of the offset vector, t, as (10)To account for different absolute scales in the maps, one normalizes the crosscorrelation function (11)where and are the means of signals in two maps, respectively, σ_{f} and σ_{g} are the standard deviations computed as, (12)for σ_{f} and equivalently for σ_{g}. The normalized crosscorrelation function has values between −1 and + 1.
For every given offset vector t, the crosscorrelation function measures the similarity (or correlation) between structures in the two maps, when the second map is shifted by t. The correlation function for a zero shift, t = 0, recovers the crosscorrelation coefficient, (13)as the centre of the crosscorrelation plane.
The position of the maximum of the crosscorrelation function in the t plane indicates the recovered displacement vector between the two maps, i.e. the applied offset for which the two structures match best. We compute the displacement vector as (14)The crosscorrelation function between two images always integrates over all scales involved in the map, not distinguishing the correlation or mutual displacement of structures at particular scales. This is addressed by the wavelet crosscorrelation.
3. Weighted wavelet crosscorrelation
3.1. Theory
To study the dependence of the correlation coefficient on the spatial scale, the two data sets are filtered on a scalebyscale basis by means of wavelets and then cross correlated at each scale (see e.g. Frick et al. 2001).
Here, we introduce the weighted wavelet crosscorrelation method to analyse the correlation between maps, f and g, weighted at each pixel by w_{f} and w_{g}, as a function of scale. For the filtering, the same formalism is exploited as for the Δvariance, i.e. Eq. (8) gives the wavelet to filter the maps on scale l through Eq. (4) to obtain the filtered maps F(x,l) and G(x,l), and the convolved total weights at each pixel, w_{F}(x,l) and w_{G}(x,l), are computed through Eq. (6).
To study the crosscorrelation of the structure in two maps, f and g, as a function of scale, we introduce the weighted wavelet crosscorrelation function, (15)where C_{F−G} is the weighted covariance (16)with (17)and equivalently for G_{w}(x,l), where and are computed from Eq. (7). The normalization is given by the standard deviation (18)of the F_{w} map. σ_{w,G}(l) is equivalently computed for G_{w}. The normalization WWCC function C_{w}(t,l) provides values between −1 and + 1.
The WWCC is therefore a threedimensional function depending on the offset vector t and the filter size l. In the centre of the offset plane, t = 0, the WWCC function provides the wavelet crosscorrelation coefficient r(l), i.e. the degree of correlation of the two data sets on scale l, (19)The position of the maximum of the WWCC in the offset plane gives the optimum offset vector (for scale l) at which the maps are best aligned. We introduce the wavelet displacement vector, (20)which defines the amplitude and direction of displacement between two maps on scale l. These can be split into the spatial displacement function, (21)where τ_{x} and τ_{y} are offsets along xaxis and yaxis, and the angular displacement function, (22)For an efficient computation of the WWCC, the convolution in Eq. (16) can be obtained through a multiplication in Fourier space when transforming the weighted functions (23)(24)where k = (k_{x},k_{y}) is the wavevector. Using the translational properties of the Fourier transform ℱ, (25)we can compute the integral for the WWCC function in Eq. (15) through the inverse Fourier transform ℱ^{1} { } i.e. (26)
3.2. Algorithm to compute the WWCC
The WWCC^{1} is computed for two images f and g and their weighting functions, w_{f} and w_{g}, through the following steps:

1.
Generate the weighted filtered maps for a given scale l, F(x,l) and G(x,l), using the convolution of f and g maps with the filter (Eqs. (4), (3) and (8)).

2.
Compute the combined waveletfiltered weights, w_{F} and w_{G} (Eq. (6)).

3.
Calculate the Δvariance (Eq. (5)).

4.
Compute the WWCC function (the degree of correlations for all possible displacements) on a given scale in Fourier domain (Eqs. (26), (23), (24)).

5.
Determine the wavelet crosscorrelation coefficient and wavelet displacement vector (Eqs. (19) and (20)–(22), respectively).

6.
Repeat the steps 1–5 for every scale, l.
4. Testing the analytic power and limitations of the weighted wavelet crosscorrelation
In this section, we test the WWCC method by applying it to various sets of welldefined artificial maps to answer three questions:

Can we determine individual characteristic scales in the two maps?

Can we reproduce a given displacement of structures at particular scales?

Can we trace a systematic change of the scale sizes between the two maps?
To address these questions, we use two different basic sets of simulated noisy maps. In one case, we assume Gaussian intensity profiles of a given size, representing individual smooth clumps. Then we have only one wellknown prominent scale in the two maps to be compared and we can test the detection of a possible scale difference and a displacement of the structures. The other set of data is given by selfsimilar fractional Brownian motion structures (fBm; Peitgen & Saupe 1988). They do not have any dominant scale, but are characterized by a powerlaw distribution of scales. They can be described by a powerlaw power spectrum of fractal structures and random phases in Fourier space. Here, we can test whether any scale dependent modifications (smoothing, displacement, ...) are recovered by the WWCC. The two test cases (circular and fBm structures) should eventually represent limiting cases for the actual observations of molecular clouds. In one extreme view, maps are described as a collection of “spherical blobs”, and in the other extreme they are described as scalefree, fully selfsimilar fractals. In practice, they typically contain both aspects, i.e. we find both selfsimilar structures and individual characteristic resolved structures.
For these test cases, we investigate the CC coefficient and displacement vector when changing the properties of the artificial clouds, such as the size of the individual structures, the spectral index of the selfsimilar scaling law, and the assumed noise level of the observations to test their sensitivity to those properties. The map size of all test data sets is 128 × 128 pixels (abbreviated as pix throughout the rest of the paper).
4.1. Structures with Gaussian intensity profiles
We test the WWCC method, for circular structures with Gaussian intensity profiles and some spatial displacement, to study the effect of the size of circular structures and the noise level in the correlation coefficient and the measured displacement vector as a function of scale.
The Gaussian intensity profile is generated with an amplitude equal to unity and width given by standard deviation σ. A weight (significance value) of unity is assigned to each data point (pixel) in the map.
Fig. 1 a) Maps of two circular Gaussian structures (σ_{1} = 10 pix and σ_{2} = 5 pix) shifted by 20 pix along yaxis. b) Observed with a simulated S/N = 5. 
In Fig. 1 we show two pairs of test maps given by circular Gaussian structures (with σ_{1} = 10 pix and σ_{2} = 5 pix and a displacement of the peak by τ_{i} = 20 pix along yaxis in the second map). As the crosscorrelation (Eqs. (10) and (15)) only considers the relative offset of structures between two maps, t, the result is invariant with respect to an exchange of negative offsets in map 1 by positive offsets in map 2. The WWCC always characterizes the mutual displacement of structures within the two considered data sets. Here, we always displace the structure in the second map relative to the first map. The top panels show the original structure representing a S/N = ∞, and the bottom panels are superimposed by white noise simulating typical observations with S/N = 5, i.e. σ_{noise} = 0.2.
Fig. 2 Maps of the two Gaussians with S/N = 5 from Fig. 1b filtered on scale of 5 pix a) and of 45 pix b). To allow for filtering in Fourier space, the maps are extended beyond the original boundaries before filtering. The extension is treated with w_{F} = 0 in the computation. 
4.1.1. Map filtering
The first step in the analysis is the wavelet convolution (Eq. (1)) filtering the maps on a given scale. The usable range of the filter sizes is inherited from the Δvariance analysis discussed in Sect. 2.1. It starts at a resolution of two pixels. Figure 2 shows the result, F(x,l) and G(x,l) for the S/N = 5 case for two selected wavelet filter sizes l = 5 pix and l = 45 pix. The filtered maps are larger than the original maps to allow for a convolution with nontruncated wavelets (see O08). The extension is treated with zero weighting in the further computation. We see that the maps filtered on small scales (5 pix) are dominated by noise, while the structures filtered on large scales (45 pix) are basically free of noise. Statistically, the noise dominates the crosscorrelation for all scales l below a critical size. This size depends on the signaltonoise level and is discussed later in this section.
Fig. 3 Δvariance spectra of the two Gaussians with S/N = ∞ from Fig. 1a. The Δvariance spectra of the large (left) and small (right) circular structures (Fig. 1a) are denoted by full and dotted lines, respectively. Vertical thick lines are used to denote the measured prominent scales of large and small circular structures, respectively. 
Fig. 4 Δvariance spectra of the two Gaussians with S/N = 5 from Fig. 1b. The Δvariance spectra of the large (left) and small (right) circular structures (Fig. 1b) are denoted by full and dotted lines, respectively. Vertical thick lines denote the measured prominent scales of large and small circular structures, respectively. 
4.1.2. The Δvariance spectrum
Computing the variance of the waveletfiltered maps for all filter sizes leads to the Δvariance spectra (; Eq. (5)). Figure 3 shows the resulting spectra for the original maps without noise and Fig. 4 shows the spectra for the case with S/N = 5. The Δvariance characterizes the amount of structure distributed on different spatial scales. The peaks of Δvariance spectra indicate the dominant structure size. For structures without additional small scale contributions, the Δvariance falls off like l^{4} below the dominant size. This is well seen in Fig. 3 for scales below about 8 pix. The increasing statistical uncertainty in the Δvariance for larger scales, due to the lower number of statistically independent entities of large scales in the maps, practically limits the use of the Δvariance analysis to prominent sizes of less than half of the map size (O08). The huge formal error bars in Fig. 3, following O08, are irrelevant here, as they characterize the counting statistics of individual structures, which are very bad for a single structure in an otherwise empty map, while every observed map typically contains much more structure.
The Δvariance detects the prominent scales of the circular structures at l_{p1} = 41 pix and l_{p2} = 18 pix (vertical lines in Fig. 3). This corresponds approximately to the diameter of the circles visible in colours in Fig. 1a, i.e. at a level above 10% of the peak intensity. For isotropic structures, the prominent scale approximately identifies the visible size of the structure (Mac Low & Ossenkopf 2000). We find a fixed relation between the prominent scale and the standard deviation of a circular structure l_{p} ≈ 4σ.
When we compute the Δvariance spectra of the same structures simulated with S/N = 5 (Fig. 4), we find a superimposed structure on scales less than 8 pix, which is completely due to noise. The noise contribution decreases with (see Bensch et al. 2001) up to ≈8 pix and becomes negligible towards larger scales as discussed for the map filtering above, leading to a Δvariance minimum at a scale of about 8 pix here. At scales above the minimum, the spectra behave identically to Fig. 3 and reach the maxima at scales of 41 pix and 18 pix.
4.1.3. The WWCC function
The WWCC map is finally computed through Eq. (26), providing the correlation for all possible displacements on a given scale. It is then used to compute the CC coefficient and displacement vector as a function of scale. The centre of the WWCC map represents the correlation of the two structures not correcting for any displacement. It gives the crosscorrelation coefficient for the given scale (Eq. (19)). The dominant offset between the two structures in the maps is measured as the displacement vector between the centre and the peak position of the WWCC function (Eq. (20)).
This is demonstrated in Fig. 5 for the pairs of maps waveletfiltered on scales of 5 pix and 45 pix from Fig. 2. The black crosses indicate the map centre, i.e. a zero displacement vector. The offset of 20 pixels in ydirection entered in the simulations is easily recovered as the location of the peak in the case of the 45pix filter. For the maps filtered on a 5 pixel scale, the uncorrelated noise structures are strong so that one cannot unambiguously distinguish the maximum of the WWCC at the correct offset from other maxima caused by the noise. As a consequence, the position of the correlation peak cannot be reliably determined in this case. This prevents the determination of the displacement vector on noisedominated scales less of than about 8 pixels.
Fig. 5 Crosscorrelation functions for the pairs of waveletfiltered maps from Fig. 2. Top panel: C_{w}(t,5 pix), bottom panel: C_{w}(t,45pix). The red crosses denote the centre of the offset plane t = 0, where one can read the wavelet crosscorrelation coefficient r(l) = C_{w}(t = 0,l). The peak of the crosscorrelation functions is displaced from the centre by τ(l) = τ_{i} as the WWCC recovers the input displacement of the structure in the second map. 
Fig. 6 Correlation coefficient r = C(τ = 0) as a function of scale for the maps from Fig. 1. a) Represents the pure Gaussians; b) the maps with noise resulting in S/N = 5. 
Crosscorrelation spectrum
The CC coefficients are extracted from the central pixel of the WWCC function (Eq. (19), crosses in Fig. 5) for all possible waveletfilter sizes, l. In Figs. 6a, b we show the dependence of the CC coefficient r(l) on the scale for the circular structures with S/N = ∞ and S/N = 5. As the two circles in the example are clearly adjacent, the crosscorrelation is negative at small scales, showing the expected anticorrelation below the mutual shift of 20 pixels and up to ~23 pix. The correlation curve has a shallow minimum at ≈15 pix and monotonically increases up to 0.6 at large scales where both structures are strongly blurred through the wavelet filter, so that they turn statistically similar. As the offset is comparable to the diameter of the smaller circle l_{p}, the coefficient remains well below unity even at large scales. In case of S/N = ∞, the anticorrelation is detected at all small scales, and in the case of S/N = 5 (Fig. 6b), the correlation vanishes at scales l ≲ 5 pix due to the uncorrelated smallscale noise in the two maps.
There are two main parameters shaping r(l): the first is the displacement between the structures, and the second is the ratio of prominent scales of these structures, l_{p2}/l_{p1}. To show the effect of the displacement on the correlation coefficient r(l), we compute the WWCC for pairs of circular structures (σ_{1} = 10 pix and σ_{1} = 5 pix) mutually displaced by offsets of 0, 5, 10, 15, and 20 pix (Fig. 7).
The correlation obviously becomes stronger on all scales if the displacement between the structures is smaller. An anticorrelation occurs whenever the mutual shift of the two structures is larger than 1/3 of the size of the bigger structure, which is almost independent of the size of the smaller Gaussian. For smaller displacements, the correlation remains positive at small scales. Without anticorrelation we always find a monotonic increase to large scales. When the offset between circular structures increases, the CC coefficient is reduced on all scales and turns to negative on small scales.
To quantify the behaviour of the correlation on small scales, we examine the changes of the CC coefficient at the smallest waveletfilter size, r(2 pix), as a function of the size ratio of the circles and their normalized displacement in Fig. 8. The structures correlate strongly if their prominent sizes are comparable and the offset between them is small. The correlation weakens with decreasing the size ratio or increasing the offset. The correlation is about zero along the line l_{p2}/l_{p1} ≈ 0.48τ_{i}/l_{p1}−0.21, and it turns to negative for larger displacements reaching a minimum at τ_{i}/l_{p1} ≈ 0.5 and l_{p2}/l_{p1} ≈ 1.
Fig. 7 Correlation coefficient as a function of scale for two circular structures (σ_{1} = 10 pix and σ_{2} = 5 pix) shifted by 0, 5, 10, 15, and 20 pix (full line, dotted, dashed, dashdotted, and dashdotdotdotted lines, respectively). The dashed vertical lines denote the prominent scale of the two circular structures. 
Fig. 8 Contour diagram of the smallscale CC coefficient, r(2 pix), as a function of prominent size ratio of circular structures (l_{p2}/l_{p1}) and displacement normalized to the largest prominent scale (τ_{i}/l_{p1}). Here we used S/N = ∞ and l_{p1} = 60 pix. 
Fig. 9 Contour diagram of the normalized crosscorrelation root l_{CC0}/l_{p1} as a function of prominent size ratio of circular structures (l_{p2}/l_{p1}) and displacement normalized to the largest prominent scale (τ_{i}/l_{p1}). S/N = ∞ and l_{p1} = 60 pix. 
Fig. 10 Displacement vector as a function of scale for the pairs of Gaussian maps from Fig. 1. a) Represents the results for pure Gaussians; b) for the maps with S/N = 5. The vectors are shown in the x−yplane for individual discrete lags indicated on the xaxis at the origin of the plotted vectors. 
We can also characterize the anticorrelation due to displacement through the parameter l_{CC0}, defined as the scale at which the correlation coefficient r(l) turns from negative to positive, i.e. r(l_{CC0}) = 0. In Fig. 9 we show the dependence of l_{CC0} on the relative displacement τ_{i}/l_{p1} and the size ratio of the Gaussians l_{p2}/l_{p1}. The scale of the crosscorrelation root depends strongly on the offset, but hardly on the size ratio of the structures. For offsets below τ_{i}/l_{p1} ≈ 0.3, no root is found as the crosscorrelation function is positive even at small filter sizes. For offsets larger than ≈0.8l_{p1}, i.e. displacements comparable to the prominent scale of the largest structure, the crosscorrelation function remains negative on all scales. At τ_{i} ≈ 0.7l_{p1}, we find l_{CC0} ≈ l_{p1}.
The spectrum of displacement vectors
Finally, we examine the spectrum of displacement vectors, τ(l), measured for all waveletfilter sizes. The displacement vector gives the coordinate of the peak of the WWCC relative to the central pixel (Eq. (20)). Figure 10 shows the recovered displacement vectors between circular Gaussian structures for S/N = ∞ and S/N = 5. In case of infinite signal to noise (Fig. 10a), the vectors are accurately recovered at scales less than the l_{p1} ≲ 40 pix. At larger scales, the displacement vector is slightly underestimated by up to two pixels. This is due to the finite map size truncating parts of the filtered circles that fall beyond the map boundaries. More and more of the filtered structure shows up beyond the map edges when going to larger waveletfilter sizes (see Fig. 2) so that for the remaining part within the map boundaries the mutual shift appears smaller than the applied offset. The coinciding finite map boundaries of both maps impose a correlation for larger waveletfilter sizes. This mimics a somewhat lower displacement of the structures and limits the applicability of the WWCC at large scales (see below), thereby affecting maps with low spatial dynamic range.
The spectrum of the displacement vectors for noisy maps (S/N = 5; Fig. 10b) shows completely random results for the noise dominated scales below 6 pixels where the correlation coefficient is close to zero. Up to the minimum of the Δvariance spectrum at 8 pixels, the displacement vectors remain unreliable. At scales between 8 pix and 12 pix, where the noise is still strong, but not dominant any more, we can recover the displacement vector with an accuracy ≲15%. Up to 12 pixels, the crosscorrelation coefficient is also dominated by noise, rather than actual structures in the map (see Fig. 6b). For all scales above 12 pixels, the displacement vector is recovered with an accuracy better than 10%.
While the finite maps size poses an upper limit to the usable scales, the observational noise thus poses a lower limit to the scales for which we can determine the correct structure offset.
4.1.4. Limiting scales
To systematically quantify the limits for the accurate determination of the spectrum of displacement vectors, we study the minimum l_{low} and maximum l_{upp} scales for which the displacement vector can be recovered with an accuracy better than 10%.
The upper limit for the scale, l_{upp}
Here, we consider the edge effects for different sizes of circular structures and different positions near the edge of the map. We use seven pairs of equal size Gaussian clouds simulated with S/N = ∞ and σ = 2.5, 5, 10, 15, 20, 25, and 30 pix (l_{p} = 8, 19, 40, 60, 80, 100, and 120 pix). We displace each pair of maps in y direction, by τ_{i} = 4,12, and 20 pix, thus, moving the structures closer to the map edges. For every given offset τ_{i}, we compute the spectra of displacement vectors for the seven pairs and determine the upper limit l_{upp} where the measured spatial displacement τ is recovered with an accuracy better than 10%. This is performed by evaluating a circle of radius δτ = 0.1 ×  τ_{i}  around the input displacement vector and testing whether the recovered vector falls into that circle.
Fig. 11 Upper limit for the displacement scale vs. prominent scale estimated for seven pairs of equal size circular structures (having σ = 2.5, 5, 10, 15, 20, 25, and 30 pix) offset by τ_{y} = 4, 12, and 20 pix. 
The maximum scale l_{upp} at which the displacement vector can be recovered with 10% accuracy depends on the truncation of the waveletfiltered circles at the map edges. In Fig. 11 we show the measured limiting scale l_{upp} for a number of offsets and prominent scale sizes. We find a general decrease of the limiting scale l_{upp} with increasing prominent structure size. For structures with prominent scales ≲1/6 of the map size (l_{p} ≲ 20 pix), the displacement vector can be accurately measured up to scale l_{upp} of about half the map size. For structures with larger prominent scales (≳50 pix) a reliable measurement of the displacement is only possible on smaller scales. The boundary effects strongly limit the usable scales. The truncation of the structure itself by the finite size of the map results in an underestimation of the displacement at large scales. Circular structures with sizes comparable to the map size (>100 pix) already fall beyond the map boundaries when offset by 12−20 pix, i.e. the offset can only be measured in a small range of scales l_{upp} ≲ 10 pix. However, these are scales that may be dominated by noise already.
To guarantee a reliable determination of the displacement, we fit the lower limit of the upper scale l_{upp} as a function of the prominent scale l_{p} by the linear relation, (27)shown as dashed line in Fig. 11. This relation can be used to constrain the l_{upp} of circular structures whenever the displacement does not shift the prominent structures off the map boundaries.
The lower limit for the scale, l_{low}
In Fig. 10b we have seen that for the S/N = 5 example the CC coefficient and displacement vector can not be recovered at scales below the scale of the minimum of the Δvariance spectrum l_{min} = 8 pix (Fig. 4).
Figure 12 shows the lowest scale, l_{low}, for which the displacement vector can be retrieved with an accuracy better than 10% as a function of the scale l_{min} for a number of different noise levels and displacements, using equal size circular structures. We find a considerable scatter of the limit for the reliable determination of the displacement vector when considering different offsets, but we can give a safe upper limit to l_{low} via (28)shown as solid line in Fig. 12.
Fig. 12 Lower limit for the displacement scale (l_{low}) as a function of the Δvariance minimum scale (l_{min}) for S/N = 2.5,5,10,25, and 50, and displacements of τ_{i} = 4,12,20 pix (black, grey, and open symbols). An upper limit to the lower scale is described by the solid line: l_{low} = 1.5 l_{min} + 1.5. 
The range l_{min} ≲ l ≲ l_{low} thus characterizes scales where the noise does no longer hide the underlying structure, as for scales l<l_{min}, but where it still significantly influences the crosscorrelation spectra and measured displacement vectors.
Fig. 13 Measured mean displacement (⟨ τ ⟩) vs. given displacement (τ_{i}) for S/N = ∞ (circles), S/N = 25 (squares), and S/N = 5 (triangles). The circles and triangles are displaced by 1 pixel from the identity line (dashed line) for a better visibility. The error bars represent 1σ error of the mean offset. 
To finally verify the reliability of the recovery of the displacement vector within the limits given by Eqs. (27) and (28), we restrict the spectrum of displacement vectors to that range when evaluating the results for 315 pairs of maps covering all combinations of Gaussian widths σ = 1, 4, 7, 10, 13, and 16 pix (l_{p} = 4, 16, 28, 40, 52, and 64 pix), input offsets of τ_{i,y} = 0,5,10,15, and 20 pix, and S/N values of ∞, 25, and 5. Figure 13 shows the measured mean displacement ⟨ τ ⟩ against the given displacement τ_{i} for the ensembles of 21 pairs with the same offset and noise level. The standard deviation of the derived displacements is very small so that the plotted error bars basically fall within the size of the symbols and are hard to be seen.
Overall we find a very good agreement with a minimal scatter, proving the method works, but a slightly overestimated displacement at τ_{i} = 0 pix for high noise (S/N = 5, triangle) and a slightly underestimated displacement for the largest offsets at all noise levels, because of the finite map size effects. The deviations fall, however, well below one pixel size. Hence, we conclude that the cutoff of the spectrum of the displacement vectors by low and upper limits allows us to recover accurate offsets, i.e. we can reliably determine the displacement vector between two structures τ(l) in the full range between l_{low} and l_{upp}.
4.2. Structures of fractional Brownian motion
In contrast to the circular Gaussian structures, which have a single welldefined prominent scale, maps of the interstellar medium often show a selfsimilar behaviour without individual prominent scales. They can be represented by the fractal structure of fractional Brownian motion maps. They are characterized by a powerlaw distribution of scales and are periodic by generation in Fourier space. We use a spectral index ζ = 3 representing a typical mean value observed in the cold interstellar medium (Falgarone et al. 2007). As for the circular Gaussian structures we evaluate how well the WWCC analysis can detect scales enhanced in one structure compared to the other and the displacement of structures at particular scales within the two maps.
4.2.1. fBm structures displaced on different scales
In real clouds, structures can be offset with respect to each other on different spatial scales. This occurs e.g. in different velocity channel maps of line observations in which the large scale structure is affected by systematic motions and the small scale structure is affected by turbulent motions; in dust emission maps at different wavelengths, where local temperature gradients create small scale displacements independent of the possible large scale structure; or in maps of different chemical tracers, where incident UV radiation from one direction creates a chemical gradient on scales not mixed by turbulent flows.
Fig. 14 fBm map with ζ = 3 (left panel) and the same map after displacing all structures on scales l ≥ 10 pix by τ_{i,x} = 10 pix and τ_{i,y} = −15 pix (right panel). This pair is to mimic an interstellar cloud structure that could be created by the superposition of small scale turbulence and a large scale velocity gradient. 
To test this, we start from an fBm map with a spectral index ζ = 3 and S/N = ∞ (Fig. 14, left panel), and shift all structures with scales larger than 10 pixels by  τ_{i}  = 18 pix (τ_{i,x} = 10 pix and τ_{i,y} = −15 pix) using the Fourier shift theorem (Eq. (25)). The resulting map is shown in Fig. 14 (right panel). The spatial shift of structures does not affect the relative contribution of structures as a function of their size, so that both maps have an identical Δvariance spectrum, shown in Fig. 15. It is characterized by a perfect power law with an exponent ζ−2 = 1, representing the fully selfsimilar scaling up to the largest scales, in which the structures are limited by the available map size.
Fig. 16 Results of the WWCC for the pair of maps from Fig. 14: a) correlation coefficient and b) displacement vector as a function of scale. 1σ error bars are given. 
Figure 16 shows the results of the WWCC for the comparison of both maps. The correlation coefficient is unity at small scales (because the structures are not offset) and gradually decreases to a minimum at 17–18 pix due to displacement by 18 pix between the structures (Fig. 16a). On large scales the structures are blurred through the wavelet filter to sizes that exceed the displacement amplitude. This leads to monotonic increase of the correlation there. The displacement vector is perfectly recovered for all scales, which is zero on scales l< 10 pix and τ_{x} = 10 pix, τ_{y} = −15 pix for larger scales (Fig. 16b).
Fig. 17 a) Original fBm map generated with S/N = 5 (left) and the same fBm map displaced by τ_{i,x} = 10 pix and τ_{i,y} = −15 pix on scales l ≥ 10 pix (right). b) Δvariance of the original and displaced fBm maps, c) correlation coefficient, and d) displacement vector as a function of scale. 1σ error bars are presented. 
Figure 17 shows the corresponding results when adding noise to the maps. The noise level of S/N = 5 appears as an increased Δvariance at small scales (l< 8 pix, panel b). It lowers the CC spectrum on scales l< 8 pix, but has no impact on the measurement of the displacement vector. As the map is filled with structures on all scales, the impact of the noise is much lower here than for the sparsely populated maps inhabiting a single Gaussian circular structure from Sect. 4.1. To ensure that we actually find a smooth transition between the two extreme cases of the single Gaussian circular structure and the fBm map, we also checked the impact of the noise on recovery of the displacement spectrum in case of multiple Gaussian structures. When we compare two maps each having three randomly located Gaussian circular structures with the same characteristics as in Fig. 1b, and measure the lower limit for the displacement scale, we obtain l_{low} = 5 pix (l_{min} = 7.7 pix), i.e. a value that is considerably smaller than that for the single Gaussian structures (l_{low} = 12 pix, see open upwards triangle in Fig. 12). For pairs of maps inhabiting 30 Gaussian structures, the impact of the noise further decreases. We obtain l_{low} = 4 pix (l_{min} = 6.3 pix) confirming that the noise dominates smaller and smaller scales if the maps are filled with more circular structures. This is in line with a negligible noise impact for the fBm maps filled with structures on all scales (Figs. 16b and 17d).
Fig. 18 Top left: fBm map (Fig. 17a, left) filtered on scale of 6 pix. Top right: the fBm map displaced on scales >10 pix (Fig. 17a, right) filtered on scale of 6 pix. Bottom left: product map generated by multiplying the intensities of the top left and top right fBm maps at each pixel (Eq. (29)). 
Identification of correlated structures
To understand the nature of the correlations quantified by the WWCC, it is useful to visually inspect the filtered maps for the individual filter scales l. In the original maps (Fig. 17a), it is almost impossible to locate individual structures that are correlated between the maps in the corresponding maps, which were waveletfiltered on the scale of 6 pix (Fig. 18 top). It may be possible to visually identify some prominent structures in which the CC spectrum showed a peak indicating many correlated structures (r(l = 6 pix) ≈ 0.6, Fig. 17c) but this is extremely difficult due to the noise contribution. An easy identification of correlated structures is possible if we visualize the integration kernel of the correlation function Eq. (10) for zero offsets τ = 0, i.e. show the product of the two maps at each pixel, (29)In the product map P(x,l) (Fig. 18, bottom panel) only relatively strong (positive or negative) features that agree between both maps show up^{2}. One can easily recognize individual small “clumps” present in both maps at the same location, which can be identified by comparing the product map with the original maps (Fig. 17a).
In Fig. 19 we repeat the experiment for the larger scale of l = 17 pix where the correlation coefficient is at minimum (Fig. 17c) because the structures are displaced by τ_{i,x} = 10 pix and τ_{i,y} = −15 pix ( τ_{i} = 18 pix, Fig. 17d). The product map of the filtered maps (Eq. (29), Fig. 19 bottom left panel) shows no structures that can be identified in the individual filtered maps or the original maps in Fig. 17a, and the amplitude of the structures in the product map is relatively small. However, if we use the recovered displacement vector at l = 17 pix to shift the second map back by the measured offset vector τ(l) and take the product of the shifted map G(x + τ(l),l) and the first map F(x,l) (top right), (30)we find that the product map (Fig. 19, bottom right) recovers all of the relatively strong (positive or negative) structures seen in the filtered maps. This allows us to localize individual correlated structures to address their shape and origin, independent of a mutual shift. In Sect. 5 we encounter a pair of observed maps of the G 333 molecular cloud with properties that are very similar to the example considered here. In the observed maps, we also find correlated structures with matching locations at small scales, but global displacements when considering large scale structures.
Fig. 19 Top left: fBm map (Fig. 17a, left) filtered on scale of 17 pix. Top right: fBm map displaced on scales >10 pix by τ_{i,x} = −10 pix and τ_{i,y} = 15 pix (Fig. 17a, right) filtered on scale of 17 pix. Bottom left: product map of two fBm maps (top left and top right). Bottom right: product map of the top left and top right maps, where the latter is reversely shifted by τ_{x} = −10 pix and τ_{y} = 15 pix (Eq. (30)). 
Fig. 20 Top left: a pure fBm map generated with S/N = ∞ and spectral index ζ = 3. Top right: a pure fBm map filtered with maximum filter of size 15 pix. Bottom left: efBm map, which is generated by superimposing the pure fBm structure (top left) and the filtered fBm structure (top right) and for brightness parameter W = 1. Bottom right: efBm map shifted by τ_{i,x} = 10 pix and τ_{i,y} = 10 pix. 
4.3. Structures of fBm clouds with enhanced scales
Pronounced scales in otherwise selfsimilar clouds may indicate special physical processes acting on those scales, therefore, giving access to important characteristics of observed maps. Being able to find and compare those scales in different maps is therefore an essential step in understanding interstellar turbulence. One process producing these enhanced scales is the opacity of partially optically thick lines. They provide a saturated picture for column densities above a specific threshold. To mimic this opacity saturation effect in simulations, we enhance spatial structures in an fBm map F(x) by smoothing it with a maximum filter described by (31)where l_{f} is the filter size. The maximum filter enhances the signal on the scale of the filter size and washes out structure on scales less than the filter size. With this approach, we introduce a prominent scale with size l_{f} into the map. This is demonstrated in Fig. 20. The top left panel shows the original fBm structure and the top right panel the result of the convolution with a maximum filter of size l_{f} = 15 pix. Structures below l_{f} pix are washed there while circles of 15 pix diameter represent the dominant structures now. This would give an unrealistic picture as the pure opacity effect is always superimposed by additional small scale variations. We construct a more realistic picture by combining the original fBm, F(x), with the scaleenhanced fBm map, ℳ_{lf}(F(x)), (32)where we introduce the inverse brightness contrast parameter W, (0 <W< 2), characterizing the contribution of the pure fBm in the total map. Then, 2−W is the relative brightness of the scaleenhanced map. For values of W< 1, the enhanced structure is brighter than the pure fBm structure, while for W> 1 it is fainter. This combination should account for the characteristics of the globally selfsimilar structure and opacity effects. The resulting fBm with enhanced scale (in the following efBm) map is shown in the bottom left panel of Fig. 20 for W = 1.
Fig. 21 Δvariance spectra of the pure fBm structure and fBm structure filtered at the scale of 15 pix by the maximum filter (full and dotted lines, respectively). 
4.3.1. Recovering the enhanced scale.
In our numerical experiment we know the size of the maximum filter, but in real observations, one first has to detect and quantify the prominent structures, i.e. the manipulation of the data in our case. Mac Low & Ossenkopf (2000) and O08 have shown that the Δvariance is an appropriate tool to detect these scales in general astrophysical data sets with irregular boundaries and variable data reliability across the maps. The Δvariance spectrum measures all prominent scales that are strong enough to create a peak in the spectrum. In a globally selfsimilar structure like our fBm (or efBm) maps, there is, however, a monotonically increasing Δvariance spectrum. Figure 21 compares the Δvariance spectra of the original fBm with the spectrum obtained for the efBm map from Fig. 20. We find no peak in the Δvariance spectrum, the underlying fBm structure dominates, but information about the filter size, l_{f}, is apparently present in the relative drop of structure variation at scales below the filter size. The convolution of the map with the maximum filter of size l_{f} = 15 pix filters out smaller scale structure. The efBm has less structure on scales ≲15 pix, while at scales larger than the size of the maximum filter the Δvariance of the original fBm is basically recovered in the efBm.
Instead of searching for a peak in the Δvariance spectrum, we therefore need a new approach to find enhanced scales by looking at the steepening of the Δvariance spectrum that is visible in Fig. 21. As an auxiliary step, we first look at the pure maximum filter, which is described by a filled circle with given diameter l_{f}.
Circular structures with constant intensity
The Δvariance spectrum of a filled circle of diameter d = 20 pix is shown in Fig. 22 as a full line. The maximum of the Δvariance falls at l_{p} ≈ 20 pix ≈ l_{f}, as predicted by O08. We verified this for filled circles with l_{f} = 4,8,12,16,20,24,28 pix.
Fig. 22 Δvariance spectrum of a filled circle of diameter 20 pix (full line) and derivative of the logarithmic Δvariance spectrum g(l) of the filled circle (dotted line) for S/N = ∞. Vertical lines denote the measured prominent scale of the filled circle at l_{p} = 21.9 pix and the critical scale l_{c} = 10.3 pix, characterizing the peak of the gradient spectrum (Eq. (34)). 
To measure the prominent scale even without clear Δvariance peak, we examine the gradient of the logarithm of the Δvariance spectrum, (33)in Fig. 22 (dotted line). The steepening of the Δvariance spectrum below the prominent scale l_{f} is reflected by a pronounced peak in the gradient spectrum. The root g = 0 corresponds to the prominent scale l_{p}. We define the critical scale as the maximum of the gradient spectrum (34)For the filled circle with 20 pixels diameter the measured critical scale is l_{c} = 10.3 pix, approximately half of the circle’s diameter.
Fig. 23 Relation between critical scales and diameter of the circles for S/N = ∞,25, and 5. The bestfit linear regression line (l_{c} ≈ 0.52 l_{p}) for S/N = ∞ is shown as solid line. 
When computing the Δvariance gradient spectra for circles of l_{f} = 4,8,12,16,20,24,28 pix (circles in Fig. 23), we find a linear relation between measured l_{c} and l_{f}(35)shown as solid line in Fig. 23.
Noisy data
To test the robustness of this approach against observational noise, we add different levels of white noise to the circle maps and compute their Δvariance gradient spectra. In noisy maps, the Δvariance spectrum at small scales is dominated by noise fluctuations (compare Figs. 4 and 3) so that the critical scale l_{c} is not directly measurable through Eq. (34). To still derive l_{c}, one needs to subtract the noise contribution from the Δvariance spectra of the contaminated circular structures, i.e. (36)The corresponding noise spectrum can be obtained by running the Δvariance analysis on the noise map, obtained e.g. from emissionfree channels in an observed spectral line cube. As we construct the noisy map in our numerical simulations by simply adding a noise map to the original map, we do not need to extract it separately here.
Using this noise subtraction, we repeated the computation of the gradient peak scale l_{c} from maps with different circle sizes and noise levels S/N = 25 (squares in Fig. 23) and S/N = 5 (triangles). We find a very good match to the noisefree results with deviations by up to at most 2 pixels induced by the noise in the data. The regression coefficient (a = 0.54 ± 0.02) for the noisy maps coincides with one for S/N = ∞ (a = 0.52 ± 0.02) within the error limits.
For observed maps the determination of the noise Δvariance may, however, be affected by uncertainties that propagate into the determination of the critical scale l_{c} if the latter falls into the noisedominated regime. Errors in the noise subtraction affect the Δvariance gradient spectrum at scales below the Δvariance minimum, l ≤ l_{min} (see e.g. Fig. 17b, l_{noise dominated} ≲ l_{min} = 5 pix). This puts a lower limit on the scale l>l_{c} = l_{min}, which can be reliably measured.
Fig. 24 Mean critical scale l_{c} measured for eight fBm maps filtered with the maximum filter of size l_{f} for S/N = ∞, 25, and 5 (circles, squares, and triangles, respectively). 1σ error bars measured in a set of ten different realizations are superimposed. 
efBm structures
In Fig. 24 we show the result of the equivalent experiments for the fBm structures with enhanced scales and an inverse brightness contrast W = 1. The efBms are generated from a fBm map with spectral index ζ = 3, which is convolved with the maximum filter of the sizes l_{f} = 5, 9, 13, 17, 21, 25, 29 pix.
For each efBm, we use the gradient of the Δvariance spectrum to measure the critical scale (Eq. (34)). Measured critical scales against maximumfilter sizes are plotted in Fig. 24. The mean critical scale and its uncertainty are estimated from ten different random realizations of efBms. The circles with error bars represent the noisefree results. The data can be described by a linear relation, (37)represented by the dashed line in Fig. 24. Within 1 pix accuracy this is identical to the simple approximation without offset from the origin l_{c} ≈ 0.52 l_{f} (in agreement with Eq. (35)), which is obtained for the circular filter, and shown as solid line in Fig. 24.
The squares and triangles in Fig. 24 show the measured critical scales for the equivalent noisy maps with S/N = 25 and S/N = 5 after applying the noise correction from Eq. (36). One can see that the squares and triangles coincide well with circles for l_{f}> 1 pix, and they can be fit by the same linear relation given by Eqs. (35) and (37) (see Fig. 24).
Fig. 25 Measured slope a against inverse brightness contrast W for efBm maps with spectral indexes ζ = 2.5,3,3.5 (full, dotted, and dashed lines, respectively). Top plot: result for S/N = ∞, bottom plot: result for S/N = 5. The data points for ζ = 3 and 3.5 (squares and triangles) are horizontally displaced by W = 0.02 and W = 0.04, respectively, from the ζ = 2.5 data points (diamonds) for better visibility. The error bars represent 1 σ variations in the statistical sample. 
We repeated the experiment for a range of parameters to verify that the relation is robust against changes of the efBm spectral index and the inverse brightness contrast W. We vary the fBm spectral index in the range of 2.5 to 3.5 typical for interstellar clouds (Falgarone et al. 2007) and brightness parameters W = 0.1,0.25,0.5,1,1.5,1.75,1.9. The previous experiment used ζ = 3 and W = 1. For each combination of ζ and W, we recover the critical scales l_{c} for l_{f} = 5, 9, 13, 17, 21, 25, 29 pix and compute the slope a of the l_{c}−l_{f} relation in the range l_{f}>l_{min} pix. To estimate the statistical uncertainty in a we used ten different random realizations so that the error is composed from the ensemble variation and the imperfection of the linear fit. Figure 25 shows the results for S/N = ∞ and S/N = 5. In case of S/N = ∞ (top panel), the slope varies in the range between 0.47 and 0.63. It tends to increase with a decreasing spectral index ζ and an increasing inverse brightness contrast W. Averaged over the full range of spectral indexes (ζ = 2.5−3.5) and inverse brightness contrast parameters (W = 0.1−1.9), we obtain a mean slope of ⟨ a ⟩ = 0.54 ± 0.03. When knowing ζ from the overall slope of the Δvariance spectrum, the gradient can be even better constrained. For the three spectral indexes we obtain ⟨ a ⟩ _{ζ = 2.5} = 0.57 ± 0.03, ⟨ a ⟩ _{ζ = 3} = 0.54 ± 0.02, and ⟨ a ⟩ _{ζ = 3.5} = 0.51 ± 0.01. These values can be used directly to measure the enhanced scale from the critical scale in the Δvariance spectrum for large S/Ns.
In case of the noisy maps (bottom panel in Fig. 25), the variation of the slope is only slightly larger for inverse brightness contrasts W ≤ 1.5, but strongly deviates from the noisefree behaviour for low contrasts of the enhanced structure, i.e. values of W ≥ 1.75. This is intuitively clear as we see less and less enhanced structure in a map if we reduce its contribution by increasing W to values close to two. If the enhanced structure is strongly diluted (W> 1.5), the efBm maps appear more like pure fBm maps with only small variations of the gradient of the so that the determination of the gradient peak l_{c}, becomes very sensitive to the noise contribution. Additional noise makes a reliable detection of the enhanced scale increasingly difficult.
Fig. 26 Gradient spectra of fBm maps generated with ζ = 3, S/N = ∞, enhanced on scale of l_{f} = 15 pix and for different inverse brightness contrast parameters W = 0.25,1,1.75 and 2 (full, dotted, dashed, and dotdashed lines, respectively). The vertical dashed line indicates the upper limit to the scale where the Δvariance slope can be measured reliably. Above that scale, the spectrum is strongly affected by boundary effects of the assumed finite map. 
The impact of the inverse brightness contrast on the Δvariance gradient is visualized for the noisefree case (S/N = ∞) in Fig. 26. It shows the gradient spectra of four efBm maps with ζ = 3, l_{f} = 15 pix, and inverse brightness contrasts W = 0.25,1,1.75,2. The case of W = 2 (dotdashed line) represents the pure fBm structure showing the constant gradient g(l) = ζ−2 = 1 for twodimensional maps (Stutzki et al. 1998) at scales up to 30 pixels (dashed vertical line in Fig. 26). The drop towards larger scales is due to the impact of the map boundary limiting the size of large structures (O08). This is consistent with our results from Sect. 4.1.4 that only prominent scales up to 64 pixels, i.e. half the map size, can be detected. To omit the boundary effects, we restrict the analysis to critical scales l ≤ 30 pix. When adding scaleenhanced structures, W< 2, we see a growing peak in the gradient spectrum at l_{c} = 8 pix. It turns sharper if we lower W, i.e. the contrast of the peak gradient g_{max} relative to the average gradient ⟨ g ⟩ grows when we increase the contribution of the scaleenhanced structures by lowering the inverse brightness contrast parameter W. The contrast of the peak value g_{max} relative to the average Δvariance gradient ⟨ g ⟩ determines whether l_{c} can be reliably determined, even if uncertainties are added to the spectrum in terms of noise.
Fig. 27 S/N = 5. Measured maximum gradient versus mean gradient for efBm maps with spectral indexes ζ = 2.5,3,3.5 (full line, dotted, and dashed lines, respectively) and different inverse brightness contrasts W = 0.1,0.25,0.5,1,1.5,1.75,1.9. The error bars indicate the standard deviation of the ensemble of ten different random realizations and seven different enhancement scales. The longdashed line is the identity representing straight spectra, i.e. g_{max} = ⟨ g ⟩. The dashdotted line represents the lower limit of g_{max} as a function of ⟨ g ⟩ below which the scale of the peak cannot be reliably determined (see Eq. (38)). 
In Fig. 27 we show the result of the systematic study of the relation between g_{max} and ⟨ g ⟩ for different values of the spectral index ζ and the inverse brightness contrast W for S/N = 5, where ⟨ g ⟩ is measured between l_{min} and 30 pixels. Averages and error bars are computed for efBms ensembles from ten different random numbers and enhanced on scales of l_{f} = 5,9,13,17,21,25,29 pix. The series of different inverse brightness contrasts W for the same spectral index ζ are connected by solid (ζ = 2.5), dotted (ζ = 3.0), and dashed (ζ = 3.5) lines. The longdashed line indicates the identity, i.e. the behaviour of pure fBms (W = 2) not showing any maximum in the gradient (dotdashed line in Fig. 26). Weakly enhanced fBm maps (W = 1.9) are positioned slightly above the identity. The deviation grows for stronger enhanced fBms, i.e. towards smaller inverse brightness contrasts W< 2.
As Fig. 25 has shown, for noisy data the scale of the steepest gradient cannot be reliably determined if the efBm is only weakly enhanced so that the gradient peak is too shallow. We can translate Fig. 27 into an easily usable criterion for the contrast of g_{max} relative to ⟨ g ⟩, which still allows for a reliable measurement of a and thus l_{f} through l_{c}. For S/N = 5, points with W ≥ 1.75 had to be excluded. This corresponds to the area below the dashdotted line in Fig. 27. It can be described by g_{max} values that fall below (38)This relation is computed by connecting the data points with W = 1.75 and adding the 3σ error margin of σ_{⟨ gmax ⟩} = 0.017 of the individual data points. All efBm structures in which the enhancement scale cannot be measured reliably due to an inverse brightness contrast that is too high (W ≳ 1.75 in Fig. 25b) fall below this relation. For W ≤ 1.5, critical scales can be reliably recovered for S/N = 5. The mean slopes obtained for S/N = ∞ and S/N = 5 (0.54 ± 0.03 and 0.51 ± 0.04) agree within the error limits.
Figure 27 can also be used to estimate spectral index and inverse brightness contrast of an efBm by measuring g_{max} and ⟨ g ⟩. For high inverse brightness contrasts W> 0.5 corresponding to about g_{max}− ⟨ g ⟩ < 0.4 spectral index and inverse brightness contrast can be uniquely determined. For lower values of W, there is an ambiguity in determination of ζ and W, but it is still possible to determine ζ with an accuracy of about 0.5.
One can generalize the approach of measuring the enhancement scale l_{f} in efBm maps (Eq. (38)) for S/N levels larger than S/N = 5. They show different thresholds of the inverse brightness contrast above which l_{f} cannot be determined reliably anymore. When lowering the noise, the threshold approaches W = 2 approximately linearly with the noise level, shifting down the dotdashed line in Fig. 26 towards the identity line. This corresponds to a change of the constant in Eq. (38) from 0.1 to 0 when S/N increases, i.e. (39)
Global fit
We can adopt the single value ⟨ a ⟩ = 0.52 ± 0.04 for estimating the enhancement scale, (40)Even without a priori knowledge of the spectral index of an efBm cloud, one can measure its enhancement scale with accuracy of about ± 8 % if the prominent structure is strong enough to meet the criterion of Eq. (39).
However, Fig. 27 can also be used to estimate spectral index, allowing for a more accurate determination of the slope a. When including noise levels from S/N = ∞ to S/N = 5 in the fit, we measure the mean slopes ⟨ a ⟩ _{ζ = 2.5} = 0.55 ± 0.04, ⟨ a ⟩ _{ζ = 3} = 0.53 ± 0.05, and ⟨ a ⟩ _{ζ = 3.5} = 0.49 ± 0.06, allowing for a more accurate determination of the enhancement scale l_{f} than through the general Eq. (40).
Altogether this gives a recipe for the measurement of a pronounced scale in a structure that is globally dominated by selfsimilarity. After applying the noise correction to the Δ variance spectrum, the Δvariance gradient spectrum has to be evaluated to measure the mean gradient ⟨ g ⟩, the peak gradient g_{max}, and the location of the peak l_{c}. Depending on the noise in the data, the user has to evaluate whether the brightness contrast of the enhanced scale of a cloud is strong enough. If the gradient peak falls above Eq. (39), i.e. g_{max}>g_{max, limit}, then it is sharp enough to allow for a reliable measurement of its position and one can use the critical scale l_{c}>l_{min} to recover the enhancement scale using the relation l_{f} = 1.92l_{c} (Eq. (40)).
4.3.2. Detecting and recovering displacements
Next, we explore the power of the WWCC to quantify the displacement between different efBm structures through the CC coefficient spectrum and the spectrum of displacement vectors. In Fig. 28 we show the CC coefficient spectrum when comparing the original fBm and the efBm map without displacement (Fig. 20, top left and bottom left panels). The structures are highly correlated on small and large scales. The scale filtering with l_{f} = 15 pix produces a small minimum on a scale of about 5 pix because of the reduction of structures below the filter size. Above the filter size both maps become very similar, leading to a crosscorrelation coefficient close to unity.
Fig. 28 Spectrum of the CC coefficient for the original fBm map and efBm map from Fig. 20 (bottom left). 
Figure 29a shows the result of the WWCC when comparing the fBm map and the efBm map displaced by τ_{i} = 14.1 pix (τ_{i,x} = 10 pix and τ_{i,y} = 10 pix, Fig. 20, top left and bottom right panels). We find a behaviour very similar to that for the displaced Gaussians in Fig. 6. The spectrum of the CC coefficients shows an anticorrelation at small scales with a minimum at ~8 pix, a steep increase from the minimum to about 30 pix, and a shallower increase at large scales. The spectrum turns to positive CC coefficients at about 14 pix approximately matching the offset amplitude. At larger scales, the correlation becomes stronger as the wavelet filter only measures structures with sizes above the enhancement and offset scale. It is evident that the displacement weakens the correlation on all scales as compared with Fig. 28. The effect is strongest at small scales, i.e. below the offset amplitude. The enhancement of the 15 pix scale in the efBm relative to the original fBm does not affect the recovery of the displacement vector (Fig. 29b). It is accurately measured over all scales l ≲ 40 pix. At larger scales, the finite map size (see Sect. 4.1.3) leads to a small underestimate of the amplitude of the displacement vector by ~5% ≤ 1 pix.
Fig. 29 Results of the WWCC for the original fBm map and the shifted efBm map from Fig. 20 (bottom right): a) correlation coefficient and b) displacement vector as a function of scale. 1σ error bars are given. 
Fig. 30 WWCC for two efBm maps (shown in a), maximumfiltered on scales of 15 pix and 5 pix) generated with a S/N = 5. The second efBm is shifted by τ_{i} = 14.1 pix (τ_{i,x} = 10 pix and τ_{i,y} = 10 pix). Part b) shows the Δvariance spectra of the first map (full line) and the second map (dotted line) with marks of critical scales (l_{c} = 6.4 pix and l_{c} = 3 pix, full and dotted vertical lines, respectively) calculated from their noisecorrected spectra; c) the correlation coefficients; and d) the measured displacement vectors as a function of scale. 
To combine all of this, we finally consider a pair of efBm maps with additional noise and an offset by τ_{i} = 14.1 pix (τ_{i,x} = 10 pix and τ_{i,y} = 10 pix, Fig. 30). The first efBm map is generated using a maximum filter of size l_{f1} = 15 pix, the second efBm map with maximum filter of size l_{f2} = 5 pix. The noise in both maps gives a S/N = 5. The maps are shown in Fig. 30a, the Δvariance spectra in 30b, the crosscorrelation spectrum in 30c, and the spectrum of detected displacement vectors in 30d. The effect of the noise is evident in the Δvariance spectra as an increase of the variance towards small scales. Below l_{min} ~ 6 pix the noise dominates, leading to a zero crosscorrelation, but it has little effect on the recovery of the displacement vectors. The change of the vector amplitude remains within a 10% accuracy. Above the noise scale the correlation curve behaves in the same way as in the case of S/N = ∞ (see Fig. 29a). The noise has no effect on r(l) at scales larger than ≈6 pix. The amplitude of the displacement vector is also slightly underestimated on large scales as in the noisefree case. The scale enhancement in both structures has basically no effect on the outcome of the WWCC. The scale enhancement is only visible in the Δvariance, where the two critical scales can be measured as indicated in Fig. 30b^{3}.
Fig. 31 Correlation coefficient as a function of scale for efBm maps filtered with maximum filter of size l_{f1} = 5 pix and l_{f2} = 15 pix and offset by 0, 5, 10, 15, and 20 pix (full line, dotted, dashed, dashdotted, and dashdotdotdotted lines, respectively). The dashed vertical lines denote the size of the filters. 
To study the quantitative impact of the displacement of the efBm maps on the CC coefficient more quantitatively, we perform the same experiment as for the Gaussians in Fig. 7, using two efBm maps filtered with maximumfilter sizes of l_{f1} = 15 pix and l_{f2} = 5 pix, and displacing them by τ_{i,y} = 0,5,10,15, and 20 pix relative to each other. The result is shown in Fig. 31. The general behaviour is qualitatively similar to Fig. 7. The shape of the CC coefficient spectrum is regulated by the offset value and ratio between the smaller to the larger filter size, l_{f2}/l_{f1}. Without any offset between the maps, we find a strong correlation between structures on all scales. It increases quickly to unity above the scale of the smallest filter size, l_{f2} = 5. If the structures are offset by 5 pix (dotted line) there is no longer any overlap below that scale so that the crosscorrelation coefficient vanishes. The global shift leads to a lower correlation on all scales, including the largest scales. With increasing the offset (dashed, dasheddotted, and dashdotdotdotted lines) the r(l) curve shifts to larger scales, a scale range of negative values (anticorrelation of filtered structures) appears, and the correlation becomes weaker on all scales. Obviously, the WWCC detects the displacement in the same way for the simple Gaussian structures in Fig. 7 and for closeto selfsimilar (e)fBm structures.
Fig. 32 Measured mean displacement (⟨ τ ⟩) vs. given displacement (τ_{i}) for S/N = ∞, 25, and 5 (filled circles, squares, and filled triangles, respectively). The circles and triangles are displaced by 1 pixel from the identity line (dashed line) for a better visibility. The error bars represent 1σ variations. 
Finally, we test how well the displacement can be recovered for pairs of maps maximumfiltered on different scales. We filter the original fBm map with maximum filters of size l_{f} = 5,9,13,17,21,25,29 pix to generate seven efBm maps with ζ = 3.0 and W = 1. Combining these seven maps (without repetition) gives 21 pairs of distinct maps. For a given pair of maps, one map is shifted by τ_{i} = 0,5,10,15,20 pix, respectively and for each shift we perform the WWCC and recover the displacement (τ; Eq. (21)) for ten random realizations of the fBm. Figure 32 shows the mean recovered displacements separately for S/N = ∞,25 and 5.
Similar to the case of the Gaussian circular structures (Fig. 13), the mean displacements ⟨ τ ⟩ are recovered with high accuracy for all noise levels and all offsets less than 1/6 of the map size (τ_{i} ≤ 20 pix) for the efBm structures also. We also tested the identity between input and recovered displacement for efBm maps generated for all combinations of the spectral index ζ = 2.5,3, and 3.5, and the inverse brightness contrast parameter W = 0.5,1,1.5 (Eq. (32)), and found a perfect agreement for all combinations of ζ and W. The errors of the measured offset depends on the parameter W. For large W the offset error slightly increases, however, it remains within the resolution limit ± 1 pix.
5. Application of WWCC to the molecular cloud G 333
We selected molecular line maps of the giant molecular cloud G 333 obtained with the Mopra telescope to test the application of the WWCC to observed maps (Lo et al. 2009). Over 20 molecular transitions were mapped and analysed through the principal component analysis (PCA) to investigate spatial correlations among different line transitions and classify molecules into high and lowdensity tracers. The PCA quantified the similarity of the different maps for eight significant principal components. Each component can be visualized and the components follow a hierarchy of sizes, but the PCA is not able to clearly identify individual spatial scales at which the similarity of different maps is broken or where gradients between the mapped structures occur. To prove the value of the WWCC in identifying these scales, we selected three of the maps from Lo et al. (2009) that show a different behaviour in the PCA. The maps of ^{13}CO 1–0 and C^{18}O 1–0 show very similar eigenvalues for the first five eigenvectors, indicating a very good correlation at most scales. The map of HCN 1–0 in contrast only shows the same eigenvalue for the first principal component, but a strongly deviating behaviour for basically all other components. Here, we try to quantify the differences and commonalities seen by the PCA for the three maps in terms of the correlation and displacement between structures in the maps as a function of their spatial scales.
To stay comparable to the results of the PCA, we follow the same procedure in producing the analysed total intensity maps as performed by Lo et al. (2009). The maps were spatially smoothed with a Gaussian of FWHM = 45′′ = 0.75 arcmin^{4} and molecular lines of ^{13}CO and C^{18}O were integrated over the velocity range from −70 to −40 km s^{1}. A wider velocity range from −80 to −30 km s^{1} was chosen in case of HCN because of visible line wings. The maps are shown in Fig. 33. At the distance of 3.6 kpc of G 333 (Lockman 1979), the resolution of 0.75 arcmin corresponds to 0.79 pc.
Fig. 33 Integrated intensity maps of ^{13}CO a), C^{18}O b) and HCN c) emission lines of the G 333 taken by Lo et al. (2009; left panels) and significance weights w for the different points in the maps (right panels). White colour in the weight map indicates a significance of unity corresponding to a median signaltonoise ratio of 25 or above. For the ^{13}CO map, only pixels close to the map boundary have a lower S/N, i.e. w< 1. 
In the next step, we need to generate significance maps (weights) for the intensity maps to account for the uncertainty in the information in the individual pixels due to observational noise, stemming from variable sensitivities and finite integration times. Ossenkopf et al. (2008b) proposed using a saturating linear function of the inverse noise level as weighting function, w = min(1,α × S/N) with α being an appropriate scaling factor. The choice of the saturation level, i.e. the S/N above which we assume that the distortion of the structural information by noise is negligible, is somewhat arbitrary. Based on our numerical experiments in the previous sections and inspection of obviously “noisy structures” in the maps, we use a value of S/N = 25 here, where we define the signal level as the median of the intensity over the map.
We estimate the noise at each pixel from the emissionfree channels in the velocity ranges from −80 to −75 km s^{1} and −27 to −15 km s^{1} for ^{13}CO and C^{18}O. For HCN, we use the velocity ranges −80 to −70 km s^{1} and −30 to −20 km s^{1}. The significance maps are given next to the integrated intensity maps in Fig. 33. Because of the high signaltonoise ratio of the ^{13}CO observations, the S/N = 25 limit means that we consider almost all the measured information in the ^{13}CO map as reliable, with the exception of a few pixels at the map boundaries that have a lower integration time coverage. For the C^{18}O and HCN maps, larger regions with low coverage producing some noisy patterns are weighted down by their lower significance in the statistical analysis of the Δvariance and the WWCC. The significance maps basically represent the coverage of the map in the mosaicing observation with multiple coverages of the individual subfields visible as square areas in the significance maps. Saturated (white) strips and areas in the maps of weights indicate very good coverage, leading to low noise so that all details of the lines can be seen. The combination of the mosaicing observations leads to a high significance (low noise) in overlapping areas and a lower significance (higher noise) at the map boundaries. To test the sensitivity of our results on the choice of the saturation limit, we varied the limit by a factor two in both directions but found no measurable impact on the Δvariance spectra and only a small impact on the WWCC on the scale of a few pixels, well within the error bars.
Fig. 34 Δvariance spectra of ^{13}CO, C^{18}O and HCN emission maps (full, dotted and dashed lines, respectively). Prominent scales of the ^{13}CO, C^{18}O and HCN maps are marked by vertical full, dotted, and dashed lines, respectively. 
Figure 34 shows the Δvariance spectra for the integrated intensity maps of ^{13}CO, C^{18}O, and HCN. The C^{18}O and HCN clouds have a dominant scale size of 7.2 and 10 arcmin (7.5 and 10.5 pc), while the ^{13}CO emission has a larger dominant structure with l_{f} ~ 12 arcmin (12.5 pc). This matches approximately the size of the largest structures with more than half of the peak intensity level in the individual maps.
Based on the results from Sect. 4.3.1, we can also estimate the enhanced scale of these maps using the critical scale l_{c} (Eq. (40)) computed from noisecorrected maps (see Appendix A for an example of the noise correction). The gradient spectra of the noisecorrected Δvariance are shown in Fig. 35 in comparison to the spectrum obtained for a pure fBm with ζ = 2.5 convolved with a Gaussian beam of 0.75 arcmin.
In the overall shape, we find a clear similarity between the spectra from the simulated map and observed maps. On small scales, there is a peak due to the blurring of smaller structures through the telescope beam with a filter size of 0.75 arcmin, as discussed already by Bensch et al. (2001). This dominates the gradient spectra below 2 arcmin. A pure Gaussian beam should provide a monotonous increase towards small scales as seen for the HCN data. The drop of the gradient spectra for the ^{13}CO and C^{18}O at the two smallest lags may be either due to an imperfect noise correction or to a relative surplus of structures at or close to the resolution limit. Therefore, we cannot reliably quantify the structural properties of the maps at scales below 1 arcmin.
Above the scales affected by the beam, we also find a significant difference between the convolved fBm and the observed maps. Instead of flat spectrum with a drop at scales approaching the map size for the fBm, the observed maps show a clear peak around 5−6 arcmin (5.5 pc) and a quick drop of the gradient towards larger scales, providing the roots that match the prominent scales of 7−12 arcmin (7−12.5 pc) discussed above. The secondary peaks in the gradient spectrum happen on critical scales ≈6.3 arcmin for ^{13}CO and HCN and ≈4.8 arcmin for C^{18}O. Using Eq. (40), this translates into enhancement scales of ≈12 arcmin (^{13}CO and HCN, 12.5 pc) and 9 arcmin (C^{18}O, 9.4 pc), differing from the measured pronounced scales of 12, 10, and 7 arcmin by at most two arcminutes, proving both methods to be approximately consistent.
We can compare the scales found by the Δvariance analysis with the results from the PCA analysis by Lo et al. (2009). The largescale distribution of the emission in all lines is traced by the first principal component (their Fig. 14), showing typical structure sizes of 5–10′, but the PCA only measures to what degree the three maps match that component. The PCA does not quantify the match or mismatch in terms of a size scale and it does not measure the difference in the dominant structure size for the three maps. The clump analysis also performed by Lo et al. (2009) only finds clumps that are much smaller, with sizes <2′.
Measurements of ⟨ g ⟩ and g_{max} of a cloud allow us to estimate the spectral index by interpolating between ζ = 2.5,3, and 3.5 (Fig. 27). In the inertial range, we expect to find ⟨ g ⟩ = ζ−2. To evaluate ⟨ g ⟩, we are restricted to the range not affected by beam smearing, i.e. to l> 3 arcmin. We use the plateau before the second peaks (Fig. 35) to estimate the spectral indices of the cloud emission structure as ζ_{C13O} = 2.8, ζ_{18CO} = 2.3, ζ_{HCN} = 2.5.
Fig. 35 Gradients of the noisecorrected Δvariance spectra (g(l)) of ^{13}CO, C^{18}O and HCN emission maps (full, dotted and dashed lines, respectively). Critical scales of the Δvariance gradients of ^{13}CO, C^{18}O, and HCN are marked by vertical full, dotted, and dashed lines, respectively. The dashdotted line represents the gradient spectrum of a pure fBm map (ζ = 2.5) convolved with a Gaussian filter of FWHM = 0.75 arcmin. 
In Figs. 36 and 37, we show the results of the application of the WWCC to the three pairs of maps, i.e. ^{13}CO and C^{18}O, ^{13}CO and HCN, and C^{18}O and HCN, in terms of the crosscorrelation coefficient spectra and spectra of displacement vectors. For the pair of ^{13}CO and C^{18}O maps the crosscorrelation coefficient shows a strong match (r(l) ≈ 0.85−0.89) for all scales >2 arcmin (Fig. 36). In spite of the apparent differences in the two maps, this confirms the strong similarity of the emission in both molecules, tracing the same conditions of interstellar gas. The difference at small scales is partially due to noise and partially optical depth effects in ^{13}CO at the densest spots in the map. The fact that the correlation does not reach unity at larger scales must be basically due to the insufficient excitation of C^{18}O in low density gas, leading to the apparently smaller size of the emitting area. To a lesser degree, this is the result of relatively small systematic displacement. The WWCC result, however proves that this effect is scaleindependent (above 2 arcmin), i.e. we find the same amount of thin gas, dark in C^{18}O, but bright in ^{13}CO on all spatial scales in the molecular cloud. This is fully in line with the fractal description of molecular clouds.
When comparing the CO isotopes with HCN, however, we find a weaker correlation on all scales and in particular a significant drop of the CC coefficient at the scale below ≈7 arcmin (7 pc). The weakest correlation is found between C^{18}O and HCN (r(l> 2 arcmin) ≈ 0.7). The increase of the CC coefficient at 8 arcmin scale is also visible here but less pronounced. This weak correlation contradicts the frequently made assumption that both species are highdensity tracers, which are sensitive to the same dense gas concentrated in small clumps and cores. As both molecules have very different critical densities our weak correlation at small scales probably reflects different excitation conditions there, i.e. a thermalization of the CO isotopes over larger scales (lower densities) compared to HCN. As all highdensity clumps are embedded in lower density envelopes, the correlation is still well above 0.5, but significantly different from unity. Possible physical reasons for kink of the CC curve at the scale of ≈7 arcmin is discussed in Sect. 5.2.
Fig. 36 Dependence of the CC coefficient on spatial scale for three pairs of emission maps, ^{13}CO and C^{18}O, ^{13}CO and HCN, and C^{18}O and HCN (full, dotted and dashed lines, respectively). 
As the PCA is based on the computation of the crosscorrelation matrix (Eq. (10)), we can directly compare our scale dependent crosscorrelation coefficients (Eq. (15), Fig. 36) with the global crosscorrelation coefficients already computed by Lo et al. (2009). They measured coefficients of 0.88, 0.79, and 0.75 for the ^{13}CO and C^{18}O, ^{13}CO and HCN, and C^{18}O and HCN maps, respectively, when comparing all pixels of their integrated intensity maps. Lo et al. (2009) did not specify the uncertainty in the coefficients, hence, we repeated their computation of the correlation coefficients and obtained errors of about 0.01. When we compare these global CC coefficients with the average of the spectrum of the CC coefficient r(l) over the full range of spatial scales, the scaleaveraged CC coefficients are slightly lower (0.82 ± 0.04, 0.75 ± 0.05, and 0.69 ± 0.05 for ^{13}CO and C^{18}O, ^{13}CO and HCN, and C^{18}O and HCN maps) than the global CC coefficients computed without weighting function. The difference is marginally significant and can be due to two effects: the inclusion of the weighting function tends to lower the CC coefficients on large scales by 0.02−0.05, and the small CC coefficients on the noisedominated scales ≲2 arcmin further reduce the average crosscorrelation coefficient. When restricting ourselves to scales without significant noise distribution, l> 2 arcmin, we obtain numbers closer to the direct correlation coefficients measured from PCA (0.85, 0.78 and 0.73). This indicates that the global crosscorrelation coefficient traces differences in the maps on scales independent from noise quite well, but it does not deal with a variable reliability of the data and it cannot distinguish between differences on different noisefree scales, such as the varying correlation with HCN below and above 7′. The WWCC method is capable of recovering the CC coefficients, also measured by the PCA, and, in addition, it allows the analysis of the CC coefficients on scalebyscale basis.
Fig. 37 Dependence of the displacement vector on spatial scale for three pairs of emission maps, ^{13}CO and C^{18}O a); ^{13}CO and HCN b); and C^{18}O and HCN c). 
Figure 37 shows the distribution of measured displacement vectors as a function of scale for the three pairs of maps^{5}. There is no displacement between the structures of ^{13}CO and C^{18}O clouds (Fig. 37 a) on small scales (≲10 arcmin), while the structure is offset at larger scales with an amplitude of ~1 arcmin, where all structures in ^{13}CO are shifted to the southwest relative to C^{18}O. If we consider the pairs with HCN, however, we find a much larger offset at large scales (Figs. 37b and c). There is a gradual increase of the offset up to ≈3.5 arcmin (HCN relative to ^{13}CO) and up to 5 arcmin (HCN relative to C^{18}O), where HCN is offset relative to the CO isotopes in southwest direction along the filament.
Fig. 38 Top panels: integrated intensity maps of C^{18}O and HCN emission lines waveletfiltered on scale of l = 5 arcmin (left and right panels, respectively). Bottom left: product map generated by multiplying the two waveletfiltered maps (top panels). 
Fig. 39 Top panels: integrated intensity maps of C^{18}O and HCN emission lines waveletfiltered on scale of l = 18 arcmin (left and right panels, respectively). Bottom left: product map generated by multiplying the two waveletfiltered maps (top panels). Bottom right: shifted product map of the top left and top right maps where the latter one is shifted by measured offset in the northeast direction (τ_{x} = −2.8 arcmin and τ_{y} = 4.5 arcmin). Note the increase of the signal for the shifted combination compared to the direct product. 
5.1. Identification of correlated structures
To understand the nature of the structures that are actually responsible for the measured shift and correlation, we go one step back and look at the individual filtered maps and compare them as we did for the fBm maps in Sect. 4.2.1. Based on the outcome of the WWCC, we examine i) structures with a scale of 5 arcmin, i.e. below the kink in the crosscorrelation spectrum at 7 arcmin; and ii) structures at a scale of 18 arcmin, i.e. showing the maximum offset between the maps, for the pair of C^{18}O and HCN maps.
Figure 38 (top panels) shows the maps waveletfiltered on scales of 5 arcmin. The correlation coefficient of the maps at this scale is about r(l = 5′) ≈ 0.7 and the offset between them is small τ(l = 5′) ≈ 0.5′. In the figure, we can identify two relatively bright cores in C^{18}O in the central region of the cloud, one core also matches a peak in HCN, while the second breaks up into two knots in HCN. The peak in the filtered HCN map is further offset to the southwest, not having any direct counterpart in C^{18}O. Multiplication of these maps (P(x,l = 5′); see Eq. (29), Fig. 38, bottom left) reveals three relatively bright correlated features at the locations of the three knots seen in HCN. In the northern core (relative RA ≈−2′, Dec ≈−2′), we find only a small shift of the HCN peak relative to the C^{18}O peak. In the southern core, we find one feature (RA ≈−7′, Dec ≈ 7′) that is prominent both in C^{18}O and HCN. The third peak (relative RA ≈ 0.3′ and Dec ≈−10′) stems from the global peak in the filtered HCN map, which has no bright counterpart in the C^{18}O map, but falls on a relatively faint elongated region there. The matching peaks dominate the crosscorrelation while the southern knot drives the measured offset. The WWCC result at small scales combines the contribution from all three features. The two matching knots, and in particular the northern core, which is brightest in C^{18}O, are very similar in both maps and have a size of ≲8 arcmin. The similarity is probably caused by warm and dense cores producing a similar radial emission profile for both transitions.
They create a crosscorrelation coefficient of about 0.7 and do not contribute to any measured offset. In the third feature, HCN is clearly offset from the C^{18}O emission. The offset hardly contributes to the crosscorrelation function, but it produces the measured small global offset.
In Fig. 39 we show the same analysis for the C^{18}O and HCN maps waveletfiltered on the scale of 18 arcmin. The WWCC showed a crosscorrelation coefficient r(l = 18′) ≈ 0.7 level and a displacement of the HCN structure by τ_{x} = 2.8 arcmin and τ_{y} = −4.5 arcmin in southwest direction relative to C^{18}O (Figs. 36 (dashed line) and 37c). The filtered maps are dominated by a cometary structure with a relatively similar shape, but a clear mutual offset. The simple product map (Fig. 39, bottom left panel) reflects this shape, but the displacement between the maps adds a negative arclike distribution in southwest direction and leads to a low amplitude of the product maps of at maximum 1.8. When accounting for the offset in shifting the HCN map by the measured displacement vector from the WWCC before computing the product map (bottom right panel), the negative arclike structure disappears, the signal becomes more concentrated in the centre of the cometary structure, and the amplitude of the product map grows to 2.1. The weakening of the correlation coefficient on large scales (Fig. 36, dashed line) can be attributed to the offset between C^{18}O and HCN structures, which progressively increases towards large scales (Fig. 37c). It becomes clear that at large scales, the WWCC is dominated by the southern core also seen at small scales. This is systematically offset between HCN and C^{18}O along the filament and shows a cometaryshape structure at that scale.
5.2. Interpretation
The Δvariance spectra show the largest difference between the ^{13}CO map and the C^{18}O map, while the HCN map exhibits an intermediate behaviour (Fig. 34). The C^{18}O map has a shallow spectrum with the smallest prominent size, i.e. a relative surplus of smallscale structures relative to the other two maps. This can be seen by eye in Fig. 33. All emission structures and, in particular, the peaks are smaller than the corresponding structures in the other two tracers. This should mainly be an optical depth effect. Following Lo et al. (2009), most clumps in the source are optically thick in ^{13}CO so that one only sees an outer so called “^{13}COphotosphere”, while C^{18}O traces the full centrallypeaked column density structure. HCN 1–0 has an intermediate optical depth. Consequently, the optical depth effects produce exactly the structure blurring discussed in Sect. 4.3. As a result, the Δvariance spectrum becomes steeper and the pronounced structures appear larger than in the underlying column density profile. The true structure is probably best traced by the C^{18}O map.
In contrast to this effect, we find a much weaker spatial correlation between the HCN map and the other two maps compared to the mutual correlation between the two CO isotopologue maps. ^{13}CO and C^{18}O emission line maps are strongly correlated above the noise scale. This is explained by the fixed relative abundance and similar excitation conditions, with a critical density of only 2 × 10^{3} cm^{3}, which lead to a match of the locations of all local features. In that sense, the opacity blurring is only a secondorder effect. The small offset of the largest large structures between ^{13}CO and C^{18}O measured in the WWCC indicates that the optical depth is somewhat higher in the south of the C^{18}O peaks compared to their northern environment, and therefore, the corresponding larger ^{13}CO emission pattern is slightly shifted to the south of the C^{18}O peaks. This means that the column density profile around the cores should have shallower decrease to the south compared to the north.
The globally lower correlation coefficient between HCN and the CO isotopologues indicates a systematically different structure on all scales. We find, in particular, a clear kink towards smaller coefficients at scales below 7 arcmin. At those scales, we see in Fig. 38 that the emission of the two main cores in the cloud is very different for HCN and C^{18}O. In the northern core (−6′, + 6′), the HCN emission is systematically shifted to the south relative to C^{18}O and, in the southern core (0, −10′), HCN even peaks at a location south of the C^{18}O that is not prominent in C^{18}O at all. This systematic difference could indicate a chemical transition or a density gradient at the measured scale of about 7 pc. The HCN emission peaks in the south of the column density peaks traced by C^{18}O could stem from an increased HCN abundance, e.g. because of UV illumination (see e.g. Fuente et al. 2005), or from an increased volume density. As HCN 1–0 has a critical density of 10^{6} cm^{3}, it traces much denser gas than the CO isotopologues. The measured scale is significantly larger than the size of individual clumps in G 333, measured by Wong et al. (2008) and Lo et al. (2009) to fall between about 0.4 and 2 pc, i.e. it must reflect a global process that affects the whole cloud. As such, a process of continued sequential starformation was proposed by Nguyen et al. (2015), which would be in line with the compression of gas by newly formed stars. Wong et al. (2008) have observed this process on a scale of 9 arcmin around G 333.60.2, the northern region in our map, but that region contributes only to a small degree to the statistics in our whole map. The inclusion of more species, which are separately sensitive either to different densities or to chemical changes produced by UV radiation from young stars, should allow us to distinguish between both effects.
The systematic offset of the HCN structures relative to structures of ^{13}CO and C^{18}O at large scales (Figs. 37b and c) can be understood from the emission filtered patterns on large scales shown in Fig. 39. The structures correlated on scales of 18 arcmin have a cometarylike structure oriented in the same northeast direction. The HCN peak at that scale sits at the head of the structure. The measured displacement vector follows the cometary structure due to the shift of the individual HCN peaks towards the southeast of the corresponding C^{18}O peaks. The combination of this structure and the derived displacement vector indicate a global anisotropy either in the density structure or in the chemical structure. A density structure that is consistent with the observations asks for a statistically higher density in the southwest compared to the northeast. This could be a global feature or a structure in which every core shows a lowdensity tail towards the northeast. This would also explain the small shift between ^{13}CO and C^{18}O due to the higher optical depths associated with higher densities in the southeast. A global anisotropy in the abundance structure asks for a preferred direction of the external UV illumination of the cloud. This is not impossible, but there is no independent observational evidence for this kind of a field from the surrounding stars.
Altogether we see that the combination of the Δvariance analysis and the WWCC allow us, in principle, to distinguish the structural effects of optical depth, excitation, and variable abundance as a function of spatial scale. For a real discrimination between the three effects, however, more data needs to be included in the analysis, covering welldefined ranges of critical densities, chemical formation conditions, and optical depths.
6. Summary
We developed the weighted waveletbased crosscorrelation (WWCC) to study the correlation and displacement between structural changes in molecular clouds as a function of scale. By inheriting the properties of the Δvariance analysis from Ossenkopf et al. (2008a), the WWCC method can use a weighting function for each data point in the map to quantify their significance or variable signaltonoise ratios. The weighting function also allows us to deal with irregular map boundaries and it permits the WWCC analysis through fast Fourier transform, which considerably speeds up the computation.
The method can be applied to observations of interstellar clouds taken in different tracers or at different velocity ranges. The WWCC measures the correlated structural changes between different maps as a function of their spatial scale. Characteristic scales where the behaviour of different tracers starts to match or deviate from each other can be interpreted, e.g. as scales of chemical or phase transitions, or driving and dissipation scales in interstellar turbulence.
We performed a series of numerical tests of the WWCC for simulated maps with welldefined spatial properties. It reveals that

For structures with a welldefined size, the spectrum of crosscorrelation (CC) coefficients strongly depends on the displacement between structures and ratio of their prominent scales. The CC spectrum turns negative on small scales if the overlapping area between the two structures becomes small compared to the area that does not overlap. The degree and scale range of the anticorrelation depends mainly on the displacement and much less on the size ratio. Beyond the scale of the mutual displacement, the correlation monotonically increases. For structures without dominant scales, the CC spectrum also traces the mutual displacement: it reaches a minimum close to the scale of the offset between the structures. In case of noisy data, the amplitude of the CC spectrum is lowered at small scales, both for correlated and anticorrelated structures.

The displacement vectors can be reliably recovered at scales dominated by actual structural information, not observational noise. For overall selfsimilar structures, independent of an enhancement of particular scales, there is always enough structural information on all scales that the displacement vector can be robustly recovered even for relatively low signaltonoise levels (S/N ≥ 5). In case of individual structures with a fixed size, the lower limit for the reliable measurement of the displacement can be estimated from the minimum of the Δvariance spectrum, l_{low} = 1.5l_{min} + 1.5 pix and the upper scale is estimated from l_{upp} = −0.38 l_{p} + 65 pix, where l_{p} is the prominent scale of the largest structure.

Mac Low & Ossenkopf (2000) showed that the Δvariance can be used to measure the scale of individual prominent structures in maps. We extended the Δvariance analysis to allow for this kind of an identification of enhanced structure scales in maps that have structure on all scales also, but with some scales being slightly more prominent than the rest. By using the logarithmic gradient of the Δvariance spectrum, we can use the scale of the steepest gradient l_{c} to measure the size of the enhanced structure l_{f} = 0.52l_{c} as long as the critical scale falls above the noise limit l_{min}.
As the results of the WWCC are sometimes nonintuitive, it can be useful to inspect the individual waveletfiltered maps to understand the origin of a varying crosscorrelation and measured displacement vectors in terms of the individual features in the maps that drive the statistical parameters. The product of the maps filtered (and shifted) on a specific scale of interest allows us to identify the locations of correlated structures and recognize their shapes.
We analysed molecular line maps (^{13}CO, C^{18}O, and HCN) of the G 333 giant molecular cloud. The Δvariance spectrum and its gradients (Eq. (40)) allow us to measure prominent scales in the maps at 12 arcmin (^{13}CO), at 7–9 arcmin (C^{18}O), and at 10–12 arcmin (HCN). For the turbulent, selfsimilar structure, covering all spatial scales, we can estimate the spectral indices of the power spectrum from the Δvariance gradient spectrum as ζ = 2.8 (^{13}CO), ζ = 2.3 (C^{18}O), and ζ = 2.5 (HCN). This indicates a gradual difference between the three maps with most smallscale structure and the smallest prominent features in the C^{18}O data and the dominance of larger structures and a relatively larger prominent structure in ^{13}CO. The HCN map shows an intermediate characteristics. All indices are lower than expected from simple Kolmogorov turbulence, but in the typical range observed in molecular line observations of other interstellar clouds (Falgarone et al. 2007).
Application of the WWCC to these molecular line maps shows that:

^{13}CO and C^{18}O emission line maps are strongly correlated above the noise scale in spite of their overall very different scaling behaviour. This is expected from a constant relative abundance, similar excitation conditions, and the higher optical depth of ^{13}CO. A fixed abundance ratio and identical excitation conditions for both species provide a match of all local features of the map, but a perfect match of all structures is prevented by the larger ^{13}CO optical depth. The later leads to a suppression of the highdensity peaks relative to ther lowerdensity environments in the intensity map so that all emission patches appear somewhat larger in ^{13}CO compared to C^{18}O. The measured 1′ offset of the large structures between ^{13}CO and C^{18}O in southern direction indicates that this optical depth effect is slightly anisotropic, as a result of a shallower density gradient to the south.

Both the HCN–^{13}CO and HCNC^{18}O correlations decrease on scales less than 7 arcmin (or 7 pc), where the maps trace different structures. On larger scales, all species trace the overall structure of the molecular cloud resulting in tighter correlations. A chemical differentiation of HCN relative to the CO isotopologues or a very different volume density structure could be the origin of those differences on scales smaller than 7 pc. The offset of the HCN structure relative to structures seen in ^{13}CO and C^{18}O measures the relative shift of the HCN emission to the south along the filament. This offset may be produced by a higher HCN abundance in the south, because of an overall anisotropic radiation field, or a somewhat higher density in that direction.
The IDL code of the WWCC method is publicly available at http://hera.ph1.unikoeln.de/~ossk/ftpspace/wwcc/
In the ideal case considered here, a recovery of the critical scale is still possible below the noiselimit scale l_{min} but for observational data, this may not be reliable any more (see Sect. 4.3.1).
The MOPRA beam at the frequency of the three lines is 36′′. The smoothing was performed by Lo et al. (2009) to allow for a uniform grid for all lines from the OTF observations and a reduced noise.
The sum of the recovered displacement vectors on large scales does not exactly add up to zero because of the finite map size. The boundary treatment tends to lead to a small underestimate of the displacement amplitudes on large scales, as was shown for the displaced Gaussian circular structures (see Fig. 10).
Acknowledgments
We thank Robert Simon and Peter Frick for valuable comments and the anonymous referee for careful reading and useful suggestions. This project was financed through DFG project number Os 177/21.
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Appendix A: Recovering the Δvariance spectrum of an observed map
To recover the enhancement scale in an efBmlike molecular cloud, we need to correct the measured Δvariance spectrum for the noise contribution of the observations. Here, we demonstrate the procedure for the G333 C^{18}O 1−0 map introduced in Sect. 5 (Fig. 33b). In a first step we measure the noise distribution across the map by integrating offline channels free of emission. To avoid the need for a radiometric correction, we integrate the noise over the same width of a velocity range that is used to integrate the line emission (Δv_{noise} = Δv_{line} = 30 km s^{1}). In the C^{18}O data cube, this is achieved by integrating the noise over the velocity ranges from −80 to −65 km s^{1} and from −35 to −20 km s^{1}. The resulting noise map is shown in Fig. A.1. In case of ^{13}CO and HCN maps, the observed spectra do not contain enough channels free of emission to select the same velocity width for integrating the noise and line emission. To correct for the smaller integration range of the noise channels, Δv_{noise}< Δv_{line}, we have to scale the integrated noise intensity radiometrically by .
Fig. A.1 Noise extracted from the C^{18}O emission line map of the GMC G 333. 
Fig. A.2 Δvariance of the observed C^{18}O emission line map (dashed line) and the noise emission across the C^{18}O map in Fig. A.1 (dotted line). Their difference represents a pure Δvariance free of the noise effect (full line). The vertical line denotes the critical scale l_{c} = 0.66 arcmin at which the pure Δvariance curve is the steepest. 1σ error bars are presented. 
In the next step, we compute the Δvariance spectra of the observed C^{18}O map and the noise map (respective dashed and dotted lines in Fig. A.2). A pure Δvariance spectrum corrected for the noise (full line) is then recovered by subtracting the Δvariances of the observed C^{18}O map and the noise. The critical scale can be measured from the gradients in the corrected Δvariance spectrum (Eq. (34)).
All Figures
Fig. 1 a) Maps of two circular Gaussian structures (σ_{1} = 10 pix and σ_{2} = 5 pix) shifted by 20 pix along yaxis. b) Observed with a simulated S/N = 5. 

In the text 
Fig. 2 Maps of the two Gaussians with S/N = 5 from Fig. 1b filtered on scale of 5 pix a) and of 45 pix b). To allow for filtering in Fourier space, the maps are extended beyond the original boundaries before filtering. The extension is treated with w_{F} = 0 in the computation. 

In the text 
Fig. 3 Δvariance spectra of the two Gaussians with S/N = ∞ from Fig. 1a. The Δvariance spectra of the large (left) and small (right) circular structures (Fig. 1a) are denoted by full and dotted lines, respectively. Vertical thick lines are used to denote the measured prominent scales of large and small circular structures, respectively. 

In the text 
Fig. 4 Δvariance spectra of the two Gaussians with S/N = 5 from Fig. 1b. The Δvariance spectra of the large (left) and small (right) circular structures (Fig. 1b) are denoted by full and dotted lines, respectively. Vertical thick lines denote the measured prominent scales of large and small circular structures, respectively. 

In the text 
Fig. 5 Crosscorrelation functions for the pairs of waveletfiltered maps from Fig. 2. Top panel: C_{w}(t,5 pix), bottom panel: C_{w}(t,45pix). The red crosses denote the centre of the offset plane t = 0, where one can read the wavelet crosscorrelation coefficient r(l) = C_{w}(t = 0,l). The peak of the crosscorrelation functions is displaced from the centre by τ(l) = τ_{i} as the WWCC recovers the input displacement of the structure in the second map. 

In the text 
Fig. 6 Correlation coefficient r = C(τ = 0) as a function of scale for the maps from Fig. 1. a) Represents the pure Gaussians; b) the maps with noise resulting in S/N = 5. 

In the text 
Fig. 7 Correlation coefficient as a function of scale for two circular structures (σ_{1} = 10 pix and σ_{2} = 5 pix) shifted by 0, 5, 10, 15, and 20 pix (full line, dotted, dashed, dashdotted, and dashdotdotdotted lines, respectively). The dashed vertical lines denote the prominent scale of the two circular structures. 

In the text 
Fig. 8 Contour diagram of the smallscale CC coefficient, r(2 pix), as a function of prominent size ratio of circular structures (l_{p2}/l_{p1}) and displacement normalized to the largest prominent scale (τ_{i}/l_{p1}). Here we used S/N = ∞ and l_{p1} = 60 pix. 

In the text 
Fig. 9 Contour diagram of the normalized crosscorrelation root l_{CC0}/l_{p1} as a function of prominent size ratio of circular structures (l_{p2}/l_{p1}) and displacement normalized to the largest prominent scale (τ_{i}/l_{p1}). S/N = ∞ and l_{p1} = 60 pix. 

In the text 
Fig. 10 Displacement vector as a function of scale for the pairs of Gaussian maps from Fig. 1. a) Represents the results for pure Gaussians; b) for the maps with S/N = 5. The vectors are shown in the x−yplane for individual discrete lags indicated on the xaxis at the origin of the plotted vectors. 

In the text 
Fig. 11 Upper limit for the displacement scale vs. prominent scale estimated for seven pairs of equal size circular structures (having σ = 2.5, 5, 10, 15, 20, 25, and 30 pix) offset by τ_{y} = 4, 12, and 20 pix. 

In the text 
Fig. 12 Lower limit for the displacement scale (l_{low}) as a function of the Δvariance minimum scale (l_{min}) for S/N = 2.5,5,10,25, and 50, and displacements of τ_{i} = 4,12,20 pix (black, grey, and open symbols). An upper limit to the lower scale is described by the solid line: l_{low} = 1.5 l_{min} + 1.5. 

In the text 
Fig. 13 Measured mean displacement (⟨ τ ⟩) vs. given displacement (τ_{i}) for S/N = ∞ (circles), S/N = 25 (squares), and S/N = 5 (triangles). The circles and triangles are displaced by 1 pixel from the identity line (dashed line) for a better visibility. The error bars represent 1σ error of the mean offset. 

In the text 
Fig. 14 fBm map with ζ = 3 (left panel) and the same map after displacing all structures on scales l ≥ 10 pix by τ_{i,x} = 10 pix and τ_{i,y} = −15 pix (right panel). This pair is to mimic an interstellar cloud structure that could be created by the superposition of small scale turbulence and a large scale velocity gradient. 

In the text 
Fig. 15 Δvariance spectra for the maps from Fig. 14. 

In the text 
Fig. 16 Results of the WWCC for the pair of maps from Fig. 14: a) correlation coefficient and b) displacement vector as a function of scale. 1σ error bars are given. 

In the text 
Fig. 17 a) Original fBm map generated with S/N = 5 (left) and the same fBm map displaced by τ_{i,x} = 10 pix and τ_{i,y} = −15 pix on scales l ≥ 10 pix (right). b) Δvariance of the original and displaced fBm maps, c) correlation coefficient, and d) displacement vector as a function of scale. 1σ error bars are presented. 

In the text 
Fig. 18 Top left: fBm map (Fig. 17a, left) filtered on scale of 6 pix. Top right: the fBm map displaced on scales >10 pix (Fig. 17a, right) filtered on scale of 6 pix. Bottom left: product map generated by multiplying the intensities of the top left and top right fBm maps at each pixel (Eq. (29)). 

In the text 
Fig. 19 Top left: fBm map (Fig. 17a, left) filtered on scale of 17 pix. Top right: fBm map displaced on scales >10 pix by τ_{i,x} = −10 pix and τ_{i,y} = 15 pix (Fig. 17a, right) filtered on scale of 17 pix. Bottom left: product map of two fBm maps (top left and top right). Bottom right: product map of the top left and top right maps, where the latter is reversely shifted by τ_{x} = −10 pix and τ_{y} = 15 pix (Eq. (30)). 

In the text 
Fig. 20 Top left: a pure fBm map generated with S/N = ∞ and spectral index ζ = 3. Top right: a pure fBm map filtered with maximum filter of size 15 pix. Bottom left: efBm map, which is generated by superimposing the pure fBm structure (top left) and the filtered fBm structure (top right) and for brightness parameter W = 1. Bottom right: efBm map shifted by τ_{i,x} = 10 pix and τ_{i,y} = 10 pix. 

In the text 
Fig. 21 Δvariance spectra of the pure fBm structure and fBm structure filtered at the scale of 15 pix by the maximum filter (full and dotted lines, respectively). 

In the text 
Fig. 22 Δvariance spectrum of a filled circle of diameter 20 pix (full line) and derivative of the logarithmic Δvariance spectrum g(l) of the filled circle (dotted line) for S/N = ∞. Vertical lines denote the measured prominent scale of the filled circle at l_{p} = 21.9 pix and the critical scale l_{c} = 10.3 pix, characterizing the peak of the gradient spectrum (Eq. (34)). 

In the text 
Fig. 23 Relation between critical scales and diameter of the circles for S/N = ∞,25, and 5. The bestfit linear regression line (l_{c} ≈ 0.52 l_{p}) for S/N = ∞ is shown as solid line. 

In the text 
Fig. 24 Mean critical scale l_{c} measured for eight fBm maps filtered with the maximum filter of size l_{f} for S/N = ∞, 25, and 5 (circles, squares, and triangles, respectively). 1σ error bars measured in a set of ten different realizations are superimposed. 

In the text 
Fig. 25 Measured slope a against inverse brightness contrast W for efBm maps with spectral indexes ζ = 2.5,3,3.5 (full, dotted, and dashed lines, respectively). Top plot: result for S/N = ∞, bottom plot: result for S/N = 5. The data points for ζ = 3 and 3.5 (squares and triangles) are horizontally displaced by W = 0.02 and W = 0.04, respectively, from the ζ = 2.5 data points (diamonds) for better visibility. The error bars represent 1 σ variations in the statistical sample. 

In the text 
Fig. 26 Gradient spectra of fBm maps generated with ζ = 3, S/N = ∞, enhanced on scale of l_{f} = 15 pix and for different inverse brightness contrast parameters W = 0.25,1,1.75 and 2 (full, dotted, dashed, and dotdashed lines, respectively). The vertical dashed line indicates the upper limit to the scale where the Δvariance slope can be measured reliably. Above that scale, the spectrum is strongly affected by boundary effects of the assumed finite map. 

In the text 
Fig. 27 S/N = 5. Measured maximum gradient versus mean gradient for efBm maps with spectral indexes ζ = 2.5,3,3.5 (full line, dotted, and dashed lines, respectively) and different inverse brightness contrasts W = 0.1,0.25,0.5,1,1.5,1.75,1.9. The error bars indicate the standard deviation of the ensemble of ten different random realizations and seven different enhancement scales. The longdashed line is the identity representing straight spectra, i.e. g_{max} = ⟨ g ⟩. The dashdotted line represents the lower limit of g_{max} as a function of ⟨ g ⟩ below which the scale of the peak cannot be reliably determined (see Eq. (38)). 

In the text 
Fig. 28 Spectrum of the CC coefficient for the original fBm map and efBm map from Fig. 20 (bottom left). 

In the text 
Fig. 29 Results of the WWCC for the original fBm map and the shifted efBm map from Fig. 20 (bottom right): a) correlation coefficient and b) displacement vector as a function of scale. 1σ error bars are given. 

In the text 
Fig. 30 WWCC for two efBm maps (shown in a), maximumfiltered on scales of 15 pix and 5 pix) generated with a S/N = 5. The second efBm is shifted by τ_{i} = 14.1 pix (τ_{i,x} = 10 pix and τ_{i,y} = 10 pix). Part b) shows the Δvariance spectra of the first map (full line) and the second map (dotted line) with marks of critical scales (l_{c} = 6.4 pix and l_{c} = 3 pix, full and dotted vertical lines, respectively) calculated from their noisecorrected spectra; c) the correlation coefficients; and d) the measured displacement vectors as a function of scale. 

In the text 
Fig. 31 Correlation coefficient as a function of scale for efBm maps filtered with maximum filter of size l_{f1} = 5 pix and l_{f2} = 15 pix and offset by 0, 5, 10, 15, and 20 pix (full line, dotted, dashed, dashdotted, and dashdotdotdotted lines, respectively). The dashed vertical lines denote the size of the filters. 

In the text 
Fig. 32 Measured mean displacement (⟨ τ ⟩) vs. given displacement (τ_{i}) for S/N = ∞, 25, and 5 (filled circles, squares, and filled triangles, respectively). The circles and triangles are displaced by 1 pixel from the identity line (dashed line) for a better visibility. The error bars represent 1σ variations. 

In the text 
Fig. 33 Integrated intensity maps of ^{13}CO a), C^{18}O b) and HCN c) emission lines of the G 333 taken by Lo et al. (2009; left panels) and significance weights w for the different points in the maps (right panels). White colour in the weight map indicates a significance of unity corresponding to a median signaltonoise ratio of 25 or above. For the ^{13}CO map, only pixels close to the map boundary have a lower S/N, i.e. w< 1. 

In the text 
Fig. 34 Δvariance spectra of ^{13}CO, C^{18}O and HCN emission maps (full, dotted and dashed lines, respectively). Prominent scales of the ^{13}CO, C^{18}O and HCN maps are marked by vertical full, dotted, and dashed lines, respectively. 

In the text 
Fig. 35 Gradients of the noisecorrected Δvariance spectra (g(l)) of ^{13}CO, C^{18}O and HCN emission maps (full, dotted and dashed lines, respectively). Critical scales of the Δvariance gradients of ^{13}CO, C^{18}O, and HCN are marked by vertical full, dotted, and dashed lines, respectively. The dashdotted line represents the gradient spectrum of a pure fBm map (ζ = 2.5) convolved with a Gaussian filter of FWHM = 0.75 arcmin. 

In the text 
Fig. 36 Dependence of the CC coefficient on spatial scale for three pairs of emission maps, ^{13}CO and C^{18}O, ^{13}CO and HCN, and C^{18}O and HCN (full, dotted and dashed lines, respectively). 

In the text 
Fig. 37 Dependence of the displacement vector on spatial scale for three pairs of emission maps, ^{13}CO and C^{18}O a); ^{13}CO and HCN b); and C^{18}O and HCN c). 

In the text 
Fig. 38 Top panels: integrated intensity maps of C^{18}O and HCN emission lines waveletfiltered on scale of l = 5 arcmin (left and right panels, respectively). Bottom left: product map generated by multiplying the two waveletfiltered maps (top panels). 

In the text 
Fig. 39 Top panels: integrated intensity maps of C^{18}O and HCN emission lines waveletfiltered on scale of l = 18 arcmin (left and right panels, respectively). Bottom left: product map generated by multiplying the two waveletfiltered maps (top panels). Bottom right: shifted product map of the top left and top right maps where the latter one is shifted by measured offset in the northeast direction (τ_{x} = −2.8 arcmin and τ_{y} = 4.5 arcmin). Note the increase of the signal for the shifted combination compared to the direct product. 

In the text 
Fig. A.1 Noise extracted from the C^{18}O emission line map of the GMC G 333. 

In the text 
Fig. A.2 Δvariance of the observed C^{18}O emission line map (dashed line) and the noise emission across the C^{18}O map in Fig. A.1 (dotted line). Their difference represents a pure Δvariance free of the noise effect (full line). The vertical line denotes the critical scale l_{c} = 0.66 arcmin at which the pure Δvariance curve is the steepest. 1σ error bars are presented. 

In the text 
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