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Table A.1
Maximum impact parameters, and thermal rate and equilibrium constants as a function of the temperature of the isotope-exchange reactions (2) and (4).
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|---|---|---|---|---|
| T∕K | bmax/Å | k2/cm3 molecule−1 s−1 | k-2/cm3 molecule−1 s−1 | K2/unitless |
| 500.00 | 5.0 | 1.4581 (− 10)(a) | 7.0643 (− 11) | 2.0641 |
| 400.00 | 5.0 | 1.2857 (− 10) | 6.0748 (− 11) | 2.1164 |
| 298.15 | 5.1 | 1.0826 (− 10) | 4.9588 (− 11) | 2.1831 |
| 200.00 | 5.0 | 0.8584 (− 10) | 3.7070 (− 11) | 2.3156 |
| 100.00 | 5.0 | 0.5750 (− 10) | 2.0655 (− 11) | 2.7842 |
| 50.00 | 4.9 | 0.3850 (− 10) | 0.9623 (− 11) | 4.0008 |
| 25.00 | 4.6 | 0.2570 (− 10) | 0.3299 (− 11) | 7.7902 |
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| T∕K | bmax/Å | k4/cm3 molecule−1 s−1 | k-4/cm3 molecule−1 s−1 | K4/unitless |
| 500.00 | 5.0 | 9.9709 (− 12) | 4.8677 (− 12) | 2.0484 |
| 400.00 | 5.0 | 8.9250 (− 12) | 4.2646 (− 12) | 2.0928 |
| 298.15 | 5.0 | 7.7400 (− 12) | 3.5854 (− 12) | 2.1588 |
| 200.00 | 5.0 | 6.3078 (− 12) | 2.7473 (− 12) | 2.2960 |
| 100.00 | 5.0 | 4.3868 (− 12) | 1.6802 (− 12) | 2.6109 |
| 50.00 | 4.9 | 3.0643 (− 12) | 0.9066 (− 12) | 3.3799 |
| 25.00 | 4.8 | 2.1578 (− 12) | 0.3448 (− 12) | 6.2581 |
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