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Fig. 4

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Restructuring resulting from on-resonance irradiation at 3.0 µm for the three 20:1 H2O:X mixtures. (a) Difference of spectra taken before and after irradiation for the 20:1 H2O:X mixtures with X = NH3 (dark red), CH4 (red) or CO2 (light red). The effect on pure pASW after a comparable irradiation is shown in black. (b) Absolute area of the changes in panel a) for the raw data (lighter traces in panel a) and the smoothed traces (darker solid lines in panel a).

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