Issue |
A&A
Volume 574, February 2015
|
|
---|---|---|
Article Number | A87 | |
Number of page(s) | 6 | |
Section | Atomic, molecular, and nuclear data | |
DOI | https://doi.org/10.1051/0004-6361/201425135 | |
Published online | 29 January 2015 |
Collision rates for electron excitation of Mg V lines⋆
Department of Physics, Clark Atlanta University, Atlanta, GA 30314, USA
e-mail: stayal@cau.edu
Received: 9 October 2014
Accepted: 26 November 2014
Aims. Transition probabilities and electron impact excitation collision strengths and rates for astrophysically important lines in Mg V are reported. The 86 fine-structure levels of the 2s22p4, 2s2p5, 2p6, 2s22p33s, 2s22p33p and 2s22p33d configurations are included in our calculations. The effective collision strengths are presented as a function of electron temperature for solar and other astrophysical applications.
Methods. The collision strengths have been calculated using the B-splineBreit-Pauli R-matrixmethod for all fine-structure transitions among the 86 levels. The one-body mass, Darwin and spin-orbit relativistic effects are included in the Breit-Pauli Hamiltonian in the scattering calculations. The one-body and two-body relativistic operators are included in the multiconfiguration Hartree-Fock calculations of transition probabilities. Several sets of non-orthogonal spectroscopic and correlation radial orbitals are used to obtain accurate description of Mg V 86 levels and to represent the scattering functions.
Results. The calculated excitation energies are in very good agreement with experiment and represents an improvement over the previous calculations. The present collision strengths show good agreement with the previously available R-matrix and distorted-wave calculations. The oscillator strengths for E1 transitions normally compare very well with previous calculations. The thermally averaged collision strengths are obtained by integrating total resonant and non-resonant collision strengths over a Maxwellian distribution of electron energies and these are presented over the temperature range log 10Te = 3.2−6.0 K.
Key words: atomic data / atomic processes / line: formation
Tables 1–4 are only available at the CDS via anonymous ftp to cdsarc.u-strasbg.fr (130.79.128.5) or via http://cdsarc.u-strasbg.fr/viz-bin/qcat?J/A+A/574/A87
© ESO, 2015
1. Introduction
Infrared and ultraviolet emission lines of Mg ions have been observed in the planetary nebula NGC 7207 (Russell et al. 1977; Grewing et al. 1978; Beckwith et al. 1984). The forbidden lines between the states of the Mg V ground 2s22p4 configuration lie in the ultraviolet (UV) part of the spectrum and the lines due to the 2s22p4–2s2p5 transitions appear in the extreme ultraviolet (EUV) spectrum of the solar corona, stellar atmospheres and other astrophysical plasmas. Electron impact excitation rates and transition probabilities are useful to determine electron temperatures and densities, ionization equilibria and for deriving elemental abundances from emission lines. The UV lines due to the forbidden 2s22p4–2s22p4
and 2s22p4
–2s22p4
transitions at 2782 Å and 1324 Å, respectively, were observed in the spectra of the Symbiotic star AG Draconis by the STIS spectrograph onboard the Hubble Space Telescope (Young et al. 2006). The intensity ratio of these Mg V UV lines is temperature and density sensitive and can be used for the diagnostic of astrophysical plasmas. The EUV line due to the allowed 2s22p4
–2s2p5
transition occurs at 276.58 Å and it has been observed by Hinode/EIS (Young et al. 2007; Brooks et al. 2009) and by SOHO/CDS. Several lines of O-like ions including Mg V lines due to 2s22p4–2s2p5 and 2s2p5
–2p61S transitions have been observed with the SERTS in the EUV spectrum of solar active regions (Thomas & Neupert 1994). The intensity ratios between the forbidden 2s22p43P–2s22p41S transition and the high-excitation transitions 2s22p33s–2s22p33p and 2s22p33p–2s22p33d of O-like ions (Kink et al. 1997) are temperature sensitive and can be used to determine physical conditions in quiet and active regions of the solar corona.
Mendoza & Zeippen (1987) reported electron excitation rates for transitions between the fine-structure 2s22p4,
and
levels from their close-coupling calculations. The LS coupled reactance matrices were transformed to intermediate coupling by ignoring the relativistic effects and by using the JAJOM program (Saraph 1972, 1978). Butler & Zeippen (1994) performed a six-state (2s22p43P, 1D, 1S, 2s2p5
,
and 2p61S) R-matrix calculation to obtain electron excitation collision strengths for O-like ions including Mg V. They also performed an algebraic transformation of LS reactance matrices to intermediate coupling. The energy levels and oscillator strengths of O-like ions have been measured using various experimental techniques. However, the electron excitation collision strengths have not yet been measured. The energy levels of Mg V have been measured by Edlen (1964), Fawcett et al. (1974), Johannesson et al. (1972), Guennou et al. (1979) and Kaufman & Artru (1980). The energy levels are compiled in NIST database1. The experimental oscillator strengths can be determined using measured lifetimes and branching ratios (Flaig & Schartner 1985). Hudson et al. (2009) reported energies for the 19 LS states and 37 fine-structure levels and oscillator strengths for the allowed transitions between the 19 LS states in both length and velocity formulations using the CIV3 code (Hibbert 1975). Tachiev & Froese Fischer (2002) and Froese Fischer & Tachiev (2004) calculated energy levels, transition rates and lifetimes using the multi-configuration Hartree-Fock (MCHF) method (Froese Fischer 2007). They included relativistic effects through the one-body and two-body Breit-Pauli operators.
Bhatia et al. (2006) reported energy levels, oscillator strengths, and collision strengths for Mg V. They performed a distorted-wave calculation and thus did not include resonances in their collision strengths. The effective collision strengths for transitions between fine-structure levels of the 2s22p4, 2s2p5, 2p6, 2s22p33s and 2s22p33p configurations in Mg V are reported by Hudson et al. (2009) from a 19-state (37 fine-structure levels) R-matrix calculation which may contain some uncertainties due to the omission of the levels of 2s22p33d configuration of n = 3 complex. The levels of 2s22p33d configuration exhibit strong mixing with lower levels. The better results can be obtained by improving the target description and by including additional levels of the 2s22p33d configuration in the close-coupling expansion. New accurate calculations of electron excitation rates in the temperature range 105 − 106 K for the UV and EUV lines are needed for applications to solar plasmas. The maximum Mg V abundance in ionization equilibrium of solar plasmas occurs at round Te = 2.8×105 K (Bhatia et al. 2006). The purpose of our work is to provide highly accurate energy levels, oscillator strengths and electron excitation effective collision strengths for astrophysical applications. We included 86 levels of the 2s22p4, 2s2p5, 2p6, 2s22p33s, 2s22p33p and 2s22p33d configurations of Mg V in our MCHF calculations of transition rates and B-spline Breit-Pauli R-matrix calculations of electron excitation collision strengths. The target levels have been accurately represented by a set of spectroscopic and correlation non-orthogonal orbitals. The inclusion of additional resonance series converging to higher excited levels can change the effective collision strengths significantly for the Mg V ion around the temperature of formation in solar plasmas.
2. Excitation energies and oscillator strengths
The terms of the 2s22p4, 2s2p5, 2p6, 2s22p33s, 2s22p33p and 2s22p33d configurations of Mg V were represented by the configuration-interaction (CI) wave functions using non-orthogonal orbitals in the MCHF approach (Froese Fischer 2007; Zatsarinny & Froese Fischer 2000). The non-orthogonal orbitals were used to describe term dependence of valence orbitals as well as correlation and relaxation effects. The non-orthogonal orbitals provide flexibility in the choice of wave functions. Each target state wave function is represented by a linear combination of configuration state functions with the same LSπ symmetry as the target state. The target state wave functions for the LSJ levels are written as a sum over different LSπ value which couple to give the total Jπ as follows, (1)We obtained 1s, 2s and 2p orbitals for the ground 2s22p4 configuration terms in the Hartree-Fock (HF) calculations. We determined excited orbitals by optimization on different sates of even and odd parties using HF and MCHF methods. Separate sets of correlation orbitals
and
(l = 0−4) were generated by optimization on the ground 2s22p43P and excited 2s2p5
states, respectively, to include all important correlation effects. The non-orthogonal orbitals were used in all main terms under consideration. In all other configurations of CI expansions a common set of orthogonal 1s, 2s, 2p, 3s, 3p and 3d orbitals was used. The CI expansions for different target states were produced using the spectroscopic and correlation orbitals in the above scheme by exciting up to three electrons to spectroscopic orbitals and up to two electrons to correlation orbitals from the basic configurations used in the description of target states. The CI expansions were reduced to a manageable size using a cut-off parameter of 0.004 for the expansion coefficients. The omission of insignificant configurations affected the relative excitation energies of the states by less than 0.1%. A total of 5179 configurations were used to represent these states. We have included all important electron correlation effects for the target states under consideration. The CI expansions were further reduced for the representation of target states in the scattering calculations to 427 configurations by using a cut-off parameter of 0.02. The absolute energy of the ground 2s22p4
level was −192.35138 au from the reduced CI expansion.
The present MCHF calculated excitation energies of the target states with 5179 configurations and with 427 configurations have been compared with the available measured values from the NIST compilation1 and other MCHF calculations of Tachiev & Froese Fischer2, Superstructure calculations of Bhatia et al. (2006) and Butler & Zeippen (1994) and CIV3 calculations of Hudson et al. (2009). The present calculation of oscillator strengths included a total of 5179 configurations in CI expansions and one-body mass, Darwin and spin-orbit operators and two-body spin-other-orbit and spin-spin operators. We included mass correction, Darwin term and spin-orbit relativistic effects in the reduced 427 configurations calculation. The agreement between our two calculations is better than 1% for most states. Our MCHF calculations show excellent agreement with the measured values and with other MCHF calculations of Tachiev & Froese Fischer2. The present calculation represents an improvement over the calculations of Bhatia et al. (2006), Hudson et al. (2009) and Butler & Zeippen (1994). Hudson et al. (2009) reported lowest 37 fine-structure levels, while Butler & Zeippen presented energies of the lowest ten levels. All other theoretical calculations used a set of the same orthogonal one-electron orbitals to represent all target states. We believe that our wave functions correctly represent the main correlation corrections, the interactions between different Rydberg series and term dependence effects.
The present oscillator strengths and transition probabilities for some E1 transitions from the states of ground 2s22p4 configuration have been compared with the CI calculations of Tachiev & Froese Fischer and Bhatia et al. in Table 2. The initial and final levels of a transition are given in Cols. 1 and 2 and in Cols. 3 and 4 we have listed the corresponding (2J + 1) values of the initial and final levels. We have presented our length values of oscillator strengths and transition probabilities in Table 2. We have used experimental energies in the calculations of oscillator strengths and radiative rates. A rather reasonable agreement between different calculations is noted. Our MCHF calculation shows somewhat better agreement with the MCHF results of Tachiev & Froese Fischer. We present oscillator strengths and transition probabilities for all E1 lines between the 86 fine-structure levels in Table 3 which is available on-line only. The relativistic effects in the structure calculations were included through the spin-orbit, spin-other-orbit, spin-spin, mass and Darwin Breit-Pauli operators in the Breit-Pauli Hamiltonian. We have presented oscillator strengths in both length and velocity formulations and transition probabilities in length form in Table 3. We have also listed the wavelength of each transition in this table. The values of oscillator strengths for intercombination lines are usually much smaller than those for the dipole-allowed transitions. The intercombination lines are produced by the spin-orbit interaction by causing mixing between different LS symmetries with the same set of quantum numbers J and π. There is normally a very good agreement between the present length and velocity forms of oscillator strengths, particularly for strong transitions with significant strengths. The ratios of the present oscillator strengths in length and velocity formulations are displayed as a function of present length oscillator strengths in Fig. 1. The two horizontal lines show a deviation of 20%. It is clear from the figure that the agreement between the present length and velocity values is within 20% or so for about 70% of the transitions. For some weaker transitions with oscillator strengths less than 0.05 the deviation between the length and velocity values is larger than 20%. To some extent it is the indication of the good quality of our wave functions used in the calculations. The ratios of present length oscillator strengths with the results of Froese Fischer & Tachiev (2004) have been shown in Fig. 2. The agreement between the two MCHF calculations is within 20% for many transitions. However, for a few transitions the two sets of results differ by about 50%.
3. Collision calculation
![]() |
Fig. 1 Ratio between the present length and velocity oscillator strengths is shown as a function of length oscillator strengths. The horizontal lines indicate 20% deviation. |
![]() |
Fig. 2 Ratio between the present length oscillator strengths and results of Tachiev & Froese Fischer is shown as a function of present length oscillator strengths. The horizontal lines indicate 20% deviation. |
We used B-spline basis for the description of continuum functions and did not impose any orthogonality constraint between continuum functions and the valence spectroscopic and correlated atomic orbitals (Zatsarinny & Tayal 2002; Zatsarinny 2006). This allowed us to avoid potential inconsistencies between the continuum and bound parts of the close-coupling expansion. We included 86 fine-structure levels arising from the terms of the 2s22p4, 2s2p5, 2p6 and 2s22p33l (l = 0−2) configurations in the close-coupling expansion. This allowed us to include channel coupling effects reasonably well between the levels of the n = 2 and n = 3 complexes. The theoretical approach and codes used in the calculation of collision strengths have been described by Zatsarinny (2006), and here we present a brief outline. The total wave function in the internal region is expanded in terms of energy-independent functions
(2)where
are channel functions formed from the multi-configurational functions of the 86 target levels and uj are the radial basis functions describing the motion of the scattering electron. The operator A antisymmetrizes the wave function and expansion coefficients aijk and bik are determined by diagonalizing the (N + 1)-electron Hamiltonian. In our calculation, the radial functions uj are expanded in the B-spline basis as
(3)and the coefficients
(which now replace aijk in Eq. (2)) are determined by diagonalizing the (N + 1)-electron Hamiltonian inside the R-matrix box that contained all bound atomic orbitals used for the description of target states. The use of non-orthogonal orbitals allows us to reduce or even to avoid the introduction of additional (N + 1)-electron terms in the R-matrix expansion. The latter may lead to extensive multi-configuration expansions, especially when correlated pseudo-orbitals are employed to improve the target states. This also allowed us to avoid the pseudo-resonance structure. The relativistic effects in the scattering calculations have been incorporated in the Breit-Pauli Hamiltonian through the use of the Darwin, mass correction and spin-orbit operators. The boundary radius of the R-matrix box was chosen to be 10.43a0 (a0 = 0.529 × 10-10 m and denotes the Bohr radius) and 61 B-splines of order 8 were used for the expansion of continuum orbitals. These parameters provide converged results for an energy range up to 50.0 Ryd. The inner solutions at the boundary of the box were matched with asymptotic solutions in the outer region. The Seaton’s STGF program as extended by Badnell (1999) has been employed to find the asymptotic solutions and collision strengths. The partial waves up to 2J = 59 were calculated in the B-spline Breit-Pauli R-matrix calculations. A top-up procedure based on the Coulomb-Bethe approximation (Burgess & Sheorey 1974) was employed to estimate the contributions for 2J larger than 59 for the dipole allowed transitions. For the non-dipole transitions we have estimated the higher partial wave contributions by assuming that the collision strengths form a geometric progression in J.
The excitation rate coefficient for a transition from state i to state f at electron temperature Te is given by (4)where gi is the statistical weight of the lower level i, ΔEif = Ef − Ei is the excitation energy and the effective collision strength γif are calculated by integrating collision strengths Ωif for fine-structure levels over a Maxwellian distribution of electron energies
(5)where Ef is the energy of incident electron with respect to the upper level f. The integration in Eq. (5) should be carried out using energy dependent collision strengths from threshold to infinity. The energy dependence of collision strengths for allowed transitions can be accounted by using numerical extrapolation technique. In the asymptotic region, the collision strengths follow a high energy limiting behavior for the dipole-allowed transitions
(6)where S is the line strength. The collision strengths vary smoothly in the high energy region and exhibit an increasing trend for dipole-allowed transitions. For the electric quadrupole or magnetic-dipole non-dipole transitions the collision strengths remain fairly constant at higher energies.
4. Collision strengths and effective collision strengths
We have plotted collision strengths for the forbidden 2s22p4–2s22p4
(2782 Å) and the dipole-allowed 2s22p4
–2s2p5
(276 Å) transitions of astrophysical importance as a function of incident electron energy in Figs. 3 and 4, respectively. The incident electron energy ranges from threshold to 50.0 Ryd and thus covers both resonant and non-resonant energy regions. The collision strengths display complex resonance structures in the closed-channels region at low incident incident electron energies. We used a fine-energy mesh of 5×10-5 Ryd in the resonance energy region to resolve many narrow resonances. The collision strengths were calculated at a total of 34 352 energy points. The resonance contributions are significantly larger and more complex for the forbidden transitions than for the allowed transitions. In the above-threshold energy region where all channels are opened, the collision strengths display smooth variation with electron energy for both forbidden and allowed transitions. Our results are compared with the distorted-wave calculation of Bhatia et al. (2006) who reported collision strengths at five electron energies of 10, 20, 30, 40 and 50 Ryd. All these energies lie in the above-threshold region where there are no resonances. The collision strengths for the forbidden 2s22p4
–2s22p4
transition (Fig. 3) slowly decrease with increasing electron energy in the above-threshold energy region and our calculation is in excellent agreement with the distorted-wave calculation. For the dipole-allowed 2s22p4
–2s2p5
transition (Fig. 4), the present collision strengths show qualitative agreement with the distorted-wave results but show some small quantitative differences. The collision strengths for the allowed transitions rise with increasing electron energy as expected. our results for the dipole-allowed 2s22p4
–2s2p5
transition are lower by about 10% on an average from the results of Bhatia et al. (2006). It may be noted that the oscillator strengths from two calculations show similar differences with our oscillator strengths being smaller than those from Bhatia et al. (see Table 2).
![]() |
Fig. 3 Collision strengths for the forbidden 2s22p4 |
![]() |
Fig. 4 Collision strengths for the allowed 2s22p4 |
![]() |
Fig. 5 Effective collision strengths for the forbidden 2s22p4 |
![]() |
Fig. 6 Effective collision strengths for the forbidden 2s22p4 |
![]() |
Fig. 7 Effective collision strengths for the allowed 2s22p4 |
We have plotted effective collision strengths for the forbidden 2s22p4–2s22p4
(1–2), 2s22p4
–2s22p4
(1–4), 2s22p4
–2s22p4
(2–5) and 2s22p4
–2s22p4
(4–5) transitions as a function of electron temperature in the range log 10Te = 3.2−6.0 K in Figs. 5 and 6. Our results have been compared with the results from previous R-matrix calculations of Hudson et al. (2009) and Butler & Zeippen (1994) and close-coupling calculation of Mendoza & Zeippen (1984). A reasonable agreement between various calculations can be noted except for the 2s22p4
–2s22p4
(2−5) transition where our results show significant differences with the calculation of Hudson et al. (2009). It may be noted that the effective collision strength for this transition is almost an order smaller compared to other transitions shown here. The resonance structures in collision strengths make significant contributions to effective collision strengths at lower temperatures. The present effective collision strengths for the allowed 2s22p4
–2s2p5
(1−7) and 2s22p4
–2s2p5
(4−9) transitions have been compared with previous R-matrix calculations of Hudson et al. (2009) in Fig. 7. The agreement between the two calculations is very good. We have presented effective collision strengths for all transitions between the lowest 86 fine-structure levels considered in our work in Table 4. The indices of lower and upper levels of a transition are given in Table 1. The results are presented at 14 electron temperatures in the range log 10Te = 3.2−6.0 K suitable for modeling of stellar and solar corona and nebular plasmas. The Table 4 is available on-line only.
5. Discussion and conclusions
The target description and the convergence of close-coupling expansion are generally two major sources of error in any close-coupling scattering calculation. A comparison of calculated excitation energies and oscillator strengths with experiments and other reliable calculations as well as the fact that we used a well tested approach, our target description should be of high quality. A sufficient number of target states in the close-coupling expansion are required to achieve convergence for the transitions of interest. The collision strengths for transitions between the lower levels of the 2s22p4, 2s2p5, 2p6, 2s22p33s and 2s22p33p configurations are well converged in our calculation. The transitions from the level of the ground 2s22p4 configuration to the levels of the 2s22p4, 2s2p5, 2p6, 2s22p33s and 2s22p33p configurations should be most accurate (10% or better). The results are somewhat less accurate (~20%) for transitions between excited levels of the above configurations. For higher levels of the 2s22p33d configuration there may be significant coupling effects from higher states and thus our results for transitions involving 2s22p33d levels may be less accurate (~25% or worse).
In conclusion, we have presented accurate oscillator strengths and effective collision strengths for Mg V lines among the 86 fine-structure levels. We used non-orthogonal orbitals for the construction of CI wave functions for target levels and for the representation of scattering functions. Our target wave functions are likely to be accurate to yield reliable collision strengths from the B-spline Breit-Pauli R-matrix scattering calculations. We have attempted to account for important physical effects such as electron correlation, relativistic, and channel coupling effects. The complex resonance series converging to several excited levels make significant contributions to collision strengths. The effective collision strengths are presented over a wide range of electron temperatures suitable for modeling of emissions from various types of astrophysical plasmas.
Acknowledgments
This research work is supported by NASA grant NNX11AB62G from the Solar and Heliophysics program.
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All Figures
![]() |
Fig. 1 Ratio between the present length and velocity oscillator strengths is shown as a function of length oscillator strengths. The horizontal lines indicate 20% deviation. |
In the text |
![]() |
Fig. 2 Ratio between the present length oscillator strengths and results of Tachiev & Froese Fischer is shown as a function of present length oscillator strengths. The horizontal lines indicate 20% deviation. |
In the text |
![]() |
Fig. 3 Collision strengths for the forbidden 2s22p4 |
In the text |
![]() |
Fig. 4 Collision strengths for the allowed 2s22p4 |
In the text |
![]() |
Fig. 5 Effective collision strengths for the forbidden 2s22p4 |
In the text |
![]() |
Fig. 6 Effective collision strengths for the forbidden 2s22p4 |
In the text |
![]() |
Fig. 7 Effective collision strengths for the allowed 2s22p4 |
In the text |
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