S. Van Loo - M. C. Runacres - R. Blomme
Royal Observatory of Belgium, Ringlaan 3, 1180 Brussel, Belgium
Received 7 September 2004 / Accepted 29 November 2004
Abstract
We present a model for the non-thermal radio emission from bright O stars, in terms
of synchrotron emission from wind-embedded shocks. The model is an
extension of an earlier one, with an improved treatment of the cooling of
relativistic electrons. This improvement limits the synchrotron-emitting
volume to a series of fairly narrow layers behind the shocks. We show that the
width of these layers increases with increasing wavelength, which has
important consequences for the shape of the spectrum. We also show that the
strongest shocks produce the bulk of the emission, so that the emergent radio
flux can be adequately described as coming from a small number of shocks, or
even from a single shock.
A single shock model is completely determined by four parameters: the position of the shock, the compression ratio and velocity jump of the shock, and the surface magnetic field. Applying a single shock model to the O5 If star Cyg OB2 No. 9 allows a good determination of the compression ratio and shock position and, to a lesser extent, the magnetic field and velocity jump.
Our main conclusion is that strong shocks need to survive out to distances of a few hundred stellar radii. Even with multiple shocks, the shocks needed to explain the observed emission are stronger than predictions from time-dependent hydrodynamical simulations.
Key words: stars: early-type - stars: mass-loss - stars: winds, outflows - radio continuum: stars - radiation mechanisms: non-thermal
In a previous paper (Van Loo et al. 2004, hereafter Paper I) we
used a phenomenological model to explain
the observed spectrum of the O5 If star Cyg OB2 No. 9. The synchrotron-emitting
electrons are assumed to be accelerated by wind-embedded
shocks, such as those produced by the instability of the radiative driving
mechanism. A power law was assumed for the momentum distribution of the
electrons and the synchrotron-emitting volume was assumed to extend to an outer
boundary
.
This approach leads to a model with a small number of
free parameters, all of which are well-determined by the fit to the
observations. Particularly, the interplay between non-thermal emission and
thermal absorption places a firm constraint on the outer boundary
.
In Paper I, the spatial distribution of the relativistic electrons was given
by a power law. This implies that the radiation is emitted by a continuous
volume extending out to
.
In the present paper, we take a closer
look at this assumption. In the shock-acceleration mechanism discussed in
Paper I (first order Fermi acceleration, Bell 1978) electrons are
accelerated to relativistic energies by making many round-trips over the shock.
Relativistic electrons are subject to a number of cooling mechanisms, most notably
inverse Compton scattering in the presence of a dense radiation field
(Chen 1992). They may therefore lose their energy rather fast when they eventually escape
downstream and move away from the shock. In this case the emission is not
expected to come from a continuous volume, but rather from a number
of (possibly thin) layers behind the shocks.
Hydrodynamical models (e.g. Runacres & Owocki 2005) of instability-generated shocks show a wide variety of shock strengths (both in velocity jump and compression ratio). We find that the strongest shocks generate most of the synchrotron emission, which means that the number of layers responsible for the observed synchrotron emission can actually be quite small.
In the following, we first (Sect. 2) derive the momentum distribution of relativistic electrons in the presence of cooling and discuss the effect on the emergent flux. In Sect. 3, we then apply a model where the emission is concentrated in a small number of thin layers to radio observations of the same star which was used in Paper I, Cyg OB2 No. 9. Finally (Sect. 4), we discuss the implications of our results and draw some conclusions.
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Electrons are accelerated to high momenta, but also lose their momentum via
different energy loss mechanisms. By taking the cooling into account, the net
momentum gain rate of the acceleration process is drastically reduced. At the
high momentum end of the spectrum, electrons are mainly cooled by the
inverse-Compton scattering of photospheric UV photons at a rate
(Rybicki & Lightman 1979)
The net momentum gain per time interval due to first order Fermi acceleration
and inverse-Compton cooling is then given by
In the absence of cooling, the acceleration of electrons through
first order Fermi acceleration results in a power law momentum distribution
(Bell 1978). When cooling is taken into account, the momentum
distribution can be quite different from the power law. Near the high
momentum cut-off, the net momentum gain goes to zero and the distribution will
deviate from a pure power law. At low momenta, however, the acceleration rate is
much higher than the cooling rate, so the momentum distribution is still a power
law. Chen (1992) showed that the spectrum including Compton cooling can
be expressed as
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Figure 1:
The cooling of relativistic electrons behind a strong shock (![]() ![]() ![]() ![]() ![]() |
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We determine the normalisation constant
by specifying the
amount of energy that goes into the relativistic electrons. Following
Ellison & Reynolds (1991), we assume that the relativistic electrons
contribute little to the overall momentum balance across a shock. This means
that the pressure of the relativistic electrons is only a small fraction (
)
of the total pressure difference. It is unlikely that
is more
than 0.05 and it could be conceivably less (Blandford & Eichler 1987;
Eichler & Usov 1993). From the Rankine-Hugoniot relations we find that
the pressure difference across the shock is
The normalisation of the momentum distribution differs from the one used in Paper I, which was based on the relativistic number density being smaller than the total electron number density. For a given momentum distribution, the total number of relativistic electrons and the total energy are of course directly related. A constraint on one implies a constraint on the other. The energy constraint is, in principle, the more stringent as it is reached well before all electrons become relativistic.
While the shock travels through the stellar wind with approximately the
terminal speed ,
the relativistic electrons will move away from the shock
front with the gas, at a significantly lower speed u2 (see Eq. (4)).
This means that outer wind electrons may well have been accelerated in the inner wind.
If the shock is at
,
the distribution of electrons at radius r, close to
,
was initially accelerated when the shock was at
Once we know where the electrons are accelerated, we only need to take into
account the cooling of the electrons. Inverse-Compton cooling, adiabatic
cooling, synchrotron cooling and Bremsstrahlung cooling can all play a rôle.
Since the observable radio emission comes from electrons with momenta of the
order 100 MeV/c (see Paper I), we will only incorporate the cooling
mechanisms which act at these momenta and higher. At high momenta, the
electrons are mainly cooled by inverse-Compton cooling which dominates over
synchrotron cooling (Chen 1992). For electrons with intermediate
momenta, the adiabatic cooling is more important than Bremsstrahlung
(Chen 1992). We will therefore include only inverse-Compton and adiabatic
cooling.
The cooling rate of the
relativistic electrons is not only dependent on the momentum of the electrons,
but also changes with distance. Since the relativistic electrons
move along with the thermal gas, we will express the cooling rate as the loss
of momentum over a distance ,
where we take
.
The cooling rate for relativistic electrons is then
given by (e.g. Chen 1992)
The above expression enables us to determine the momentum
distribution after cooling.
We assume that a shock is spherically symmetric, i.e. that it covers a
complete solid angle.
The number of relativistic electrons initially having
a momentum between
and
at a radius
is then
,
with
N(p) the differential number distribution given by Eq. (10)
and
the volume that contains the electrons.
Inverse-Compton and adiabatic losses reduce the momentum of the electrons to
values between p and
where p is given by
Eq. (16). Also, the volume of the shell expands to
.
Since the number of electrons in this momentum interval and
volume is not changed, the number distribution after cooling
is given
by
An example for the momentum distribution is given in
Fig. 1. Here we plot the momentum distribution at the shock
front for a strong shock (
and
)
at
600 R* and the momentum distributions which are found 1.5 R*, 3.0 R*
and 4.5 R* behind the shock. These distributions were accelerated respectively
at 470 R*, 339 R* and 209 R*. It is clear that the highest attainable
momentum drops off rather rapidly behind the shock: electrons which are 4.5 R*behind the shock no longer contribute to the observable radio emission, i.e.
the emission layer is no thicker than 4.5 R*.
Equations (16) and (17) are valid
for both reverse and forward shocks.
The momentum distribution at a distance
behind a reverse
or forward shock is initially accelerated at
.
Electrons with a momentum
at
are then cooled down to a momentum p at r. Although r is not the same for a
reverse and forward shock, the momentum p is not significantly different as long
as
.
Since this criterion is fulfilled for
,
this means that a reverse and forward shock will have the same momentum distribution
at a distance
downstream of the shock. It is therefore possible
to discuss only forward shocks in the rest of the paper without loss of generality.
Although the emissivity is calculated by integrating over all momenta, only
electrons within a narrow range of momenta contribute to the emissivity at
a given frequency. A relativistic electron with momentum p emits most of
its energy in a narrow region around the frequency
(Ginzburg & Syrovatskii 1965)
The width of the synchrotron emission layer
is
determined by the time
to cool the relativistic electrons
below radio emitting momenta. From Eq. (15) we see that
the cooling rate decreases with distance from the star. This means that the
relativistic electrons are cooled faster close to the star and that the width
of the emission layer behind the shock is larger further out in the wind. The width
is proportional to
.
The cooling time
in principle also depends on the value of the high momentum cut-off
,
but this
turns out to be a minor effect. Furthermore, the width of the emission layer is
influenced by the outflow speed of the relativistic electrons. Because the
relativistic electrons flow away from the shock with a velocity u2 given
in Eq. (4), the width of the emission layer is directly proportional
to u2.
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Figure 2: The emissivity behind a strong forward shock at r=600 R* for 2 different wavelengths. The dashed line is the emissivity at 20 cm and the solid line at 2 cm. We normalised the emissivity to the highest value. |
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An important point is that the width of the emission layers depends on wavelength. At short wavelengths the radiation is produced by more energetic electrons (Eq. (19)). Since these electrons are cooled more rapidly by inverse-Compton cooling (Fig. 1), the emission layers at shorter wavelengths are narrower, as can be seen in Fig. 2. These differences change the shape of the synchrotron spectrum (Sect. 2.6). The emission layers in Fig. 2 are somewhat larger than expected from Fig. 1, because the emission at a given wavelength is produced by electrons, not with one specific momentum, but within a narrow momentum range.
The synchrotron radio fluxes emitted behind a shock given in Eq. (20)
can be calculated numerically. In the code (which is similar to the one used
in Paper I), the momentum integral of the emissivity, given in Eq. (18),
is computed using the trapezoidal rule and the step size is refined until it reaches
a desired fractional precision of 10-3. The emissivity has to be calculated
at different positions behind the shock. Then, the spatial integral of the
flux, Eq. (20), is treated in the same way as the momentum integral, but
up to a precision of order 1%. Here the function
is determined using a linear interpolation between precalculated values.
The number distribution is given by Eq. (17), while
the mean synchrotron power of a single electron
is determined
using precalculated values in the same way as
.
We included
the Razin effect in the calculation of
(see Paper I). The low momentum cut-off
is assumed
,
while the high momentum cut-off
is
found by evaluating Eqs. (8) in (16).
The total emergent flux also has a contribution from free-free emission by thermal electrons. This contribution is calculated using the Wright & Barlow formalism (Wright & Barlow 1975) and added to the non-thermal flux.
The normalisation constant
of the momentum distribution is
proportional to the pressure difference
across the shock, which
has a
-dependence. This means that the number of electrons in all
momentum ranges increases with the shock velocity jump. Furthermore the synchrotron
emissivity
,
given by Eq. (18), is directly proportional
to
which means that the emissivity must be proportional to
.
In
Sect. 2.3 we showed that the width of the emission layer
is also proportional to
.
From Eq. (21) it then follows that
the synchrotron flux is proportional to
.
This relation remains
valid if we use the exact expression Eq. (20) to calculate the
synchrotron flux.
The radio fluxes do not only increase with the shock velocity jump,
but also with the compression ratio .
The slope of
the momentum distribution becomes shallower with higher
(see Eq. (10)). Assuming that the
number of relativistic electrons is the same near p0 (i.e.
independent
of
), more electrons are then present in the momentum range important
for observable radio emission.
As the emissivity at a given wavelength is related to the number
of electrons with a specific momentum, more emission is radiated by the
strongest shocks. A complication arises because the normalisation constant
actually decreases with
(Sect. 2.1), thereby slightly counteracting
the effect of the slope. However, this complication turns out to have a minor effect.
A grid of models (discussed in Sect. 3.2) shows that the flux only fails to increase
with increasing
if the shock is close to the stellar surface and if at the same
time the magnetic field is strong. Even in such cases the effect is limited
to 20% on the flux.
Thus, the shocks with the highest compression ratios and shock velocity jumps in the wind dominate the radio emission.
For a power-law momentum distribution of relativistic electrons with index n, the synchrotron emissivity
is given by a power law in frequency with an
exponent (Rybicki & Lightman 1979)
In astrophysical applications the measured radio spectral index
is often used to estimate the compression ratio of the shock that accelerated
the relativistic electrons (e.g. Chen & White 1994). If we observe
synchrotron emission with a radio spectral index
then
for a non-cooling model we would derive a compression ratio
using
and Eq. (11). However, taking into account
cooling behind the shock, we find that the observed flux corresponds to
a strong shock with
.
In Paper I we applied the continuous model to the non-thermal radio emitter
Cyg OB2 No. 9 (O5 If). Of all the observational radio data that are available
for Cyg OB2 No. 9, we used the 1984 Dec. 21 observation with the VLA
(Bieging et al. 1989) because of its detection of emission in three
radio wavelength bands and the small error bars on the detection. However
the error bars on the Cyg OB2 No. 9 observations listed by Bieging et al. (1989) are surprisingly small (0.1 mJy). The error due to the
flux calibration should already be 5% of the observed flux for 2 cm
observations and 2% for 6 and 20 cm observations (Perley &
Taylor 2003), which translates to 0.29, 0.15 and
0.10 mJy at 2, 6 and 20 cm. We can therefore conclude that only the
random errors (root-mean-square) were listed. If we include the
calibration errors (absolute flux scale errors), we find:
mJy (2 cm),
mJy (6 cm) and
mJy (20 cm).
Table 1: Relevant stellar parameters for Cyg OB2 No. 9 adopted in this paper. The numbers are taken from Bieging et al. (1989, BAC), Leitherer (1988, L) and Herrero et al. (1999, HCVM).
A significant fraction of the radio emission is not radiated as synchrotron
radiation by relativistic electrons, but is due to free-free emission from
the stellar wind (Wright & Barlow 1975). Using the values from Table
1, the contributions
of the free-free emission to the observations of Cyg OB2 No. 9 are: 1.4 mJy
(2 cm), 0.7 mJy (6 cm) and 0.4 mJy (20 cm), if we assume that the stellar wind
is completely ionised. The stellar parameters adopted are listed in
Table 1. We will now apply a layered shock model to these
observations of Cyg OB2 No. 9.
Once a choice is made for the model parameters, we can calculate the
synchrotron flux in the three wavelengths for a grid in ,
,
and B* and select those combinations of the parameters that
fit the VLA observations within the error bars.
The emergent flux for one such model is shown in Fig. 3.
All possible combinations of
,
,
and B* are shown in Figs. 4a and 4b.
Strong constraints are produced on all four parameters. In principle
the ranges of the model parameters depend on p0, but we checked that
the effect is minimal.
The reason that we find strong shocks is as follows. The emission at
2 and 6 cm is barely influenced by the free-free absorption or
the Razin effect (see below). In a simple analysis, this means that,
at these wavelengths, the exponent
of the synchrotron emissivity
is simply the radio spectral index
.
We can then derive the compression ratio
of the shock directly from the radio spectrum. Using
Eqs. (11) and (22), we then find
.
(Note that this means that weaker shocks produce a steeper spectrum.) However,
the steepening due to the wavelength dependence of the emission layer (see Sect. 2.6) is not included in the above expression. This means that
the compression ratio derived for a layered model will be larger than the
compression ratio derived in the simple analysis above.
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Figure 3: The VLA observations (21 Dec. 1984) for Cyg OB2 No. 9 with revised error bars. The solid line represents a single shock model that explains the non-thermal radio emission. The stellar parameters are given in Table 1. |
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The shock responsible for the observed emission at 20 cm must be located at a
large distance from the star, due to the large
free-free absorption in the wind. All radio emission emitted too close
to the star is absorbed and cannot be observed. This absorbing volume extends
up to the radius
where the radial free-free optical depth is unity.
Using
with
the free-free absorption coefficient given by Allen (1973),
we find
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The tight constraint on
presented here is only valid
for a single shock. In Sect. 3.4, we will explain the
observations by multiple shocks. These can be spread out over a fairly large
geometric region, and the shock positions are then much
less well determined than in the case of a single shock.
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Figure 4:
a) Left panel: the combinations of ![]() ![]() ![]() ![]() |
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The reason for the tight relation is the direct dependence of the emission on
both
and B*. In the absence of the Razin effect, the
synchrotron emissivity
produced by a power-law momentum distribution is proportional to
(Rybicki & Lightman 1979). In a lower magnetic field,
the relativistic electrons emit less synchrotron radiation and the number of
electrons must increase (through
)
to produce the same emission.
Because
and
are nearly constant for all solutions (see
Fig. 4a),
can only be increased by increasing
the shock velocity jump
.
All our solutions have
,
so to first order the synchrotron
flux
(see Fig. 4b). This
largely explains the tight relation. The small difference for B*<200 G
is due to the Razin effect.
The reason why we needed
for the multiple shock model (as opposed to
for the single shock model) is that free-free absorption partly counteracts the
steepening effect of the emission layer. This is because
the free-free absorption at 2 and 6 cm is no longer
negligible for emission produced close to the star. For example, a shock near 100 R*only contributes to the 2 cm flux and not to the 6 and 20 cm flux. A consequence is that
the resulting spectrum of a multiple shock model is flatter than for a single shock model.
This means that, to produce the observed spectrum, multiple shocks must be weaker than
derived in the single shock model.
The above analysis shows that we can bring down the required velocity jump by introducing a large number (in this case 219) of shocks. This assumes that all shocks have equal strength. If the shocks have a range of strengths, the strongest shocks will dominate (Sect. 2.5), and the emergent flux will be produced only by relatively small number of strong shocks. This would make it more difficult to bring the typical velocity jump down to a value consistent with hydrodynamical results. Whether the observed spectra can be reproduced by a model based on hydrodynamical predictions will be investigated in a subsequent paper (Van Loo et al. 2005).
For magnetic fields lower than 200 G, the shock velocity jump
derived in the single shock
model is higher, hereby increasing the number of shocks needed to produce the observed
fluxes. For
the number of shocks (with
)
needed
is about 1000.
Obviously such a high number is irreconcilable with hydrodynamical models.
In the layered model there are no weak solutions (as can be seen in
Fig. 4a, ), which is an effect of
the cooling on the radio spectral index. To explain this, let us consider
the example of a multiple shock model given in Sect. 3.4.
This layered model fits the observations. It is also, to a good approximation,
a continuous model in the sense that a large part of the wind is filled
with relativistic electrons, with a fraction that is constant throughout the wind.
Yet a true continuous model with the same parameters cannot fit the observations.
The layered model has a steeper slope than the continuous model, because of
the wavelength dependence of the width of the layer. Thus the weak shock solutions
that were found in the continuous model cannot occur in the layered model.
For most solutions in the continuous model the fraction of relativistic
electrons increases further out in the wind. This means that the bulk of the
synchrotron emission is produced at the outside of the synchrotron emitting
region as it is in a single shock model. The extent of the synchrotron emitting
region
in the continuous model is also comparable to the position
of a single shock in the layered model. For B*=100 G,
is
between
520-750 R*. Therefore the continuous model and the layered model
agree on the location of the emission layer in the wind.
In this paper we refined the model from Paper I to take into account the cooling of the relativistic electrons and the large variety of shock strengths in the stellar wind. The cooling reduces the emitting volume to narrow layers behind the shock. Since the strongest shocks dominate the synchrotron emission produced, only a small number of layers are responsible for the observed flux. We further simplified the layered model by assuming that only one shock is present in the wind. Applied to a specific observation of Cyg OB2 No. 9, the model produces meaningful constraints on all parameters. The high values that we find for the shock velocity jump (compared to hydrodynamical models) suggest emission by multiple shocks. Note that there is an apparent contradiction between the large number of shocks needed to reduce the velocity jump and the small number of shocks expected to produce the bulk of the emission.
An important result of the single shock model is that the compression
ratio (
)
and the position of the shock (
)
are
well constrained. This means that strong shocks must survive up to large distances
in the wind
(a conclusion also reached by Chen 1992).
This is consistent with the results from Paper I and from
hydrodynamical calculations (Runacres & Owocki 2005). The
shock velocity jump
and the surface magnetic field B* both have values which are not so well constrained and extend over a large
range. However, these values are tightly related, so that the detection limit on B* gives a lower limit on
.
The synchrotron emission is produced by the strongest shocks in the stellar wind. Because these shocks move through the wind, the radio spectrum must change in time. This may explain the variability observed in non-thermal emitters (Bieging et al. 1989). In that case, the time-scales of the variability should be comparable to the flow time. When a single shock travels from 450 R* to 550 R*, the synchrotron emission at 20 cm increases from 0 to 4.4 mJy within a flow time of about 6 days. Therefore the time-scale of variability in Cyg OB2 No. 9 should be of the order of days to a week. However, it is unlikely that a shock would cover a complete solid angle, as it will probably be disrupted by lateral instabilities (e.g. Rayleigh-Taylor). This will reduce the amplitude of variability. Furthermore, when the synchrotron emission is produced by multiple shocks, the variations due to the changing positions of the shocks could be completely averaged out.
The efficiency of inverse-Compton and adiabatic cooling prevents electrons from carrying their energy very far from a shock. This however does not mean that the relativistic electrons need to be accelerated in situ. For example, electrons accelerated near 300 R* still emit a significant amount of synchrotron radiation by the time they reach 600 R* (see on Fig. 2 the emissivity at 597 R* produced by electrons originally accelerated at 339 R*). Thus synchrotron emission is still produced far out in the wind even though shocks do not need to survive up to these distances.
The presence of relativistic electrons in the wind also leads to the generation
of non-thermal X-rays, due to the inverse-Compton scattering of photospheric UV photons
(e.g. Chen & White 1991). Since there is an abundant supply of UV photons
near the stellar surface, the non-thermal X-ray emission is strongest in the
inner wind where there is no observable radio emission.
The emission shows up as
a hard tail in the X-ray spectrum. Since the energy of the X-ray photons (E) is
related to the energy of the incident UV photons (E0) as
(see Rybicki & Lightman 1979), with
the Lorentz factor of the
scattering electron, electrons with momenta between 10-20 MeV/c (
)
are responsible for the emission between 1-10 keV. Since the non-thermal radio
emission comes from electrons with momenta of order
,
the
non-thermal X-ray emission comes from less
energetic electrons than the non-thermal radio emission.
Even so, the non-thermal X-ray emission is dominated by the strongest shocks. In this regard
the conclusion by Rauw et al. (2002) that the compression ratio derived from the
X-ray data is
,
is somewhat surprising.
In order to produce non-thermal radio emission, only a magnetic field and relativistic electrons are required. Although a magnetic field and shocks to accelerate electrons should both be present in any early-type star, not all these stars are non-thermal emitters. A possible explanation is the value of the magnetic field. In a low magnetic field less radiation is produced by the relativistic electrons and the contribution of the synchrotron emission to the radio flux would be negligible. This suggests that the thermal emitters have a lower surface magnetic field than the non-thermal emitters (Bieging et al. 1989).
The values found for
in the single shock model are rather
high when compared to values derived from hydrodynamical models, especially
because these high values are needed far out in the stellar wind.
If we re-interpret the emission as coming from multiple shocks, the
shock velocity jump does not have to be as high as for a single shock.
For shocks in the outer wind, a shock velocity jump of
is
a reasonable value (e.g. Runacres & Owocki 2005). For
the observations are then produced by a reasonable number of shocks. In weaker fields,
however, too many shocks are required (also, the Razin effect is stronger).
Our synchrotron models will be confronted with
hydrodynamical calculations in a subsequent paper.
Both the high
value and the location of the shock at 600 R*in a single shock model
can be interpreted as coming from a colliding wind binary. The synchrotron emission is then produced by
relativistic electrons accelerated, not in wind-embedded shocks, but in a colliding-wind
shock (Eichler & Usov 1993). Even though the present model is not appropriate
for colliding winds,
the position of the shock and the value of
are close to those found
in WR 147 (Dougherty et al. 2003). This means that, although there is no spectroscopic
evidence for binarity, the observed non-thermal emission of Cyg OB2 No. 9 is consistent with
a colliding-wind binary. For Wolf-Rayet stars, the relation between non-thermal
radio emission and binarity is firmly established (Dougherty & Williams 2000).
For O stars, the situation is less clear. About half of the non-thermal O stars are
apparently single. However, recent spectroscopic studies show that one of
the archetypical single non-thermal O stars, Cyg OB2 No. 8A, is in
fact a binary (De Becker et al. 2004). Therefore, the possibility that
Cyg OB2 No. 9 is a binary cannot be excluded.
Acknowledgements
We thank S. Dougherty and J. Pittard for careful reading of the manuscript. We thank the referee, R. White, for suggestions that improved the paper. S.V.L. gratefully acknowledges a doctoral research grant by the Belgian Federal Science Policy Office (Belspo). Part of this research was carried out in the framework of the project IUAP P5/36 financed by Belspo.