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Table A.1

List of obs. and obs.−cal. transition frequencies.

N K a K c J F 1 F a v b   obs. c obs.-cal.d N K a K c J F 1 F a v b   obs. c obs.-cal.d
514−505 5.5−5.5 5−5 1 197464.267(70) 0.124 11110−11011 11.5−11.5 11−11 1 327765.463(60) 0.000
5.5−5.5 6−6 1 197466.208(100) 0.114 11.5−11.5 12−12 1 327768.371(50) 0.058
615−606 6.5−6.5 6−6 1 210920.459(60) -0.084 10.5−10.5 11−11 1 328301.285(50) 0.042
6.5−6.5 7−7 1 210922.652(60) -0.004 10.5−10.5 10−10 1 328304.694(50) 0.008
716−707 7.5−7.5 7−7 1 227328.350(60) -0.077 11.5−11.5 11−11 10−10 0 328029.021(80) -0.139
7.5−7.5 8−8 1 227330.620(60) -0.076 11.5−11.5 12−12 11−11 0 328031.528(100) -0.417
6.5−6.5 7−7 1 227659.877(60) 0.096 11.5−11.5 11−11 11−11 0 328031.528(100) 0.054
6.5−6.5 6−6 1 227662.665(100) -0.135 11.5−11.5 11−11 12−12 0 328032.285(90) -0.104
7.5−7.5 7−7 6−6 0 227604.358(80) -0.025 11.5−11.5 12−12 12−12 0 328034.237(90) -0.020
7.5−7.5 8−8 7−7 0 11.5−11.5 12−12 13−13 0 328035.236(90) 0.003
7.5−7.5 7−7 7−7 0 227606.141(80) 0.097 10.5−10.5 11−11 12−12 0
7.5−7.5 7−7 8−8 0 227606.141(80) -0.147 10.5−10.5 10−10 11−11 0
7.5−7.5 8−8 8−8 0 227608.306(80) 0.065 10.5−10.5 11−11 11−11 0
7.5−7.5 8−8 9−9 0 227608.306(80) -0.239 10.5−10.5 10−10 10−10 0
817−808 8.5−8.5 8−8 1 246966.022(60) -0.031 10.5−10.5 11−11 10−10 0
8.5−8.5 9−9 1 246968.468(60) -0.008 10.5−10.5 10−10 9−9 0 328572.325(60) 0.013
7.5−7.5 8−8 1 247341.946(60) 0.715* 12111−12012 12.5−12.5 12−12 1 362557.079(60) -0.055
7.5−7.5 7−7 1 247345.254(60) 0.906* 12.5−12.5 13−13 1 362560.063(80) -0.037
8.5−8.5 8−8 7−7 0 247239.960(60) 0.045 11.5−11.5 12−12 1 363151.666(60) -0.039
8.5−8.5 9−9 8−8 0 247242.263(60) -0.020 11.5−11.5 11−11 1 363155.152(60) -0.092
8.5−8.5 8−8 9−9 0 247242.263(60) -0.024 12.5−12.5 13−13 13−13 0 362820.961(120) -0.138
8.5−8.5 8−8 8−8 0 12.5−12.5 13−13 14−14 0 362822.137(80) 0.041
8.5−8.5 9−9 9−9 0 247244.234(60) 0.110 11.5−11.5 12−12 13−13 0 363406.389(80) 0.025
8.5−8.5 9−9 10−10 0 247244.668(60) -0.032 11.5−11.5 11−11 12−12 0 363409.756(80) -0.077
918−909 9.5−9.5 9−9 1 270103.657(60) 0.003 11.5−11.5 12−12 12−12 0 363409.756(80) 0.254
9.5−9.5 10−10 1 270106.240(60) 0.012 11.5−11.5 11−11 11−11 0 363413.087(80) 0.128
8.5−8.5 9−9 1 11.5−11.5 12−12 11−11 0 363414.369(80) -0.014
8.5−8.5 8−8 1 11.5−11.5 11−11 10−10 0 363417.898(80) -0.016
9.5−9.5 9−9 8−8 0 270374.935(100) 0.076 13112−13013 13.5−13.5 13−13 1
9.5−9.5 10−10 9−9 0 270377.474(90) 0.099* 13.5−13.5 14−14 1 401343.878(120) 0.080
9.5−9.5 9−9 9−9 0 270377.474(90) 0.590* 12.5−12.5 13−13 1 401994.391(120) 0.129
9.5−9.5 9−9 10−10 0 270377.474(90) -0.122* 12.5−12.5 12−12 1
9.5−9.5 10−10 10−10 0 808−717 8.5−7.5 8−7 7−6 1 321683.266(80) 0.048
9.5−9.5 10−10 11−11 0 8.5−7.5 8−7 9−8 1 321684.490(80) -0.182
8.5−8.5 9−9 10−10 0 270795.456(80) -0.484* 8.5−7.5 8−7 8−7 1 321684.490(80) 0.070
8.5−8.5 8−8 9−9 0 270798.448(80) -0.656* 8.5−7.5 9−8 8−7 1 321684.490(80) 0.123
8.5−8.5 9−9 9−9 0 270798.448(80) -0.314* 8.5−7.5 9−8 10−9 1 321685.704(80) -0.262
8.5−8.5 8−8 8−8 0 270801.464(80) -0.446* 8.5−7.5 9−8 9−8 1 321685.704(80) 0.120
8.5−8.5 9−9 8−8 0 270802.655(80) -0.347* 7.5−6.5 8−7 9−8 1 321831.092(120) 0.014
8.5−8.5 8−8 7−7 0 270805.852(80) -0.360* 7.5−6.5 8−7 8−7 1 321832.757(120) 0.046
1019−10010 10.5−10.5 10−10 1 296978.021(60) 0.003 7.5−6.5 7−6 8−7 1 321832.757(120) 0.165
10.5−10.5 11−11 1 296980.826(60) 0.090 7.5−6.5 7−6 7−6 1 321834.312(120) 0.140
9.5−9.5 10−10 1 297456.630(65) 0.007 7.5−6.5 8−7 7−6 1 321835.778(120) -0.037
9.5−9.5 9−9 1 297459.944(65) -0.016 7.5−6.5 7−6 6−5 1 321837.260(120) -0.180
10.5−10.5 10−10 9−9 0 297245.907(60) 0.036 909−818 9.5−8.5 9−8 8−7 1
10.5−10.5 10−10 10−10 0 297248.203(90) 0.151 9.5−8.5 9−8 10−9 1 386458.220(80) -0.043
10.5−10.5 11−11 10−10 0 297248.841(90) 0.312 9.5−8.5 9−8 9−8 1 386458.220(80) -0.029
10.5−10.5 10−10 11−11 0 297248.841(90) -0.053 9.5−8.5 10−9 9−8 1 386458.220(80) -0.034
10.5−10.5 11−11 11−11 0 297250.625(80) -0.079 9.5−8.5 10−9 11−10 1 386459.395(60) -0.033
10.5−10.5 11−11 12−12 0 297251.685(70) 0.080 9.5−8.5 10−9 10−9 1 386459.395(60) 0.101
9.5−9.5 10−10 11−11 0 8.5−7.5 9−8 10−9 1 386611.859(60) -0.028
9.5−9.5 9−9 10−10 0 297723.876(60) -0.265 8.5−7.5 9−8 9−8 1 386613.207(60) -0.034
9.5−9.5 10−10 10−10 0 297723.876(60) 0.064 8.5−7.5 8−7 9−8 1 386613.207(60) -0.011
9.5−9.5 9−9 9−9 0 297727.035(60) -0.038 8.5−7.5 8−7 8−7 1
9.5−9.5 10−10 9−9 0 297728.193(150) -0.050 8.5−7.5 9−8 8−7 1 386616.182(60) 0.025
9.5−9.5 9−9 8−8 0 297731.646(150) 0.079 8.5−7.5 8−7 7−6 1 386617.609(60) 0.012

Notes.

(a)

For para-CH2OH, the F quantum number does not exist.

(b)

The lower tunnelling state is given.

(c)

Observed frequencies (in MHz) with their estimated error measurement given in parentheses applies to the last digits. Unresolved (blended) transitions were fitted with their averaged frequencies.

(d)

Lines with an (obs.−cal.) value higher than 1.9 times their error measurement were rejected from the fit and are marked with a ∗.

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