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A&A 399, 553-565 (2003)
DOI: 10.1051/0004-6361:20021813
Turbulent diffusion and mixing in interstellar dark clouds with adsorption onto grains
C. J. Yate and T. J. MillarDepartment of Physics, UMIST, PO Box 88, Manchester M60 1QD, UK
(Received 17 April 2002 / Accepted 6 December 2002 )
Abstract
This paper reports the results of models of dark cloud chemistry
incorporating a depth dependent density distribution with diffusive mixing
and adsorption onto grains.
The model is based on the approach taken by Xie et al. (1995), with
the addition of grain accretion effects.
Without diffusion, the central regions of the cloud freeze out in less than
107 years.
Freeze-out time is dependent on density, so the diffuse outer region of the
cloud remains abundant in gas for about an order of magnitude longer.
We find that fairly small amounts of diffusive mixing can delay freeze-out
at the centre of the model cloud for a time up to an order of magnitude
greater than without diffusion, due to material diffusing inward from the
edges of the cloud.
The gas-phase lifetime of the cloud core can thus be increased by up to an
order of magnitude or more by this process.
We have run three different grain models with various diffusion coefficients
to investigate the effects of changing the sticking parameters.
Key words: astrochemistry -- turbulence -- diffusion -- ISM: abundances -- ISM: dust, extinction
Offprint request: T. J. Millar, Tom.Millar@umist.ac.uk
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